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Search Publications by: Daniel A Fischer (Fed)

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Displaying 26 - 50 of 231

A practical superconducting-microcalorimeter X-ray spectrometer for beamline and laboratory science

May 16, 2017
Author(s)
William B. Doriese, Peter Abbamonte, Douglas A. Bennett, Edward V. Denison, Yizhi Fang, Daniel A. Fischer, Colin P. Fitzgerald, Joseph W. Fowler, Johnathon D. Gard, Gene C. Hilton, Cherno Jaye, Jessica L. McChesney, Luis Miaja Avila, Kelsey M. Morgan, Young Il Joe, Galen C. O'Neil, Carl D. Reintsema, Fanny Rodolakis, Daniel R. Schmidt, Hideyuki Tatsuno, Jens Uhlig, Leila R. Vale, Joel N. Ullom, Daniel S. Swetz
We describe a series of microcalorimeter X-ray spectrometers designed for a broad suite of measurement applications. The chief advantage of this type of spectrometer is that it can be orders of magnitude more efficient at collecting X-rays than more

Magnetic Field Landscapes Guiding the Chemisorption of Diamagnetic Molecules

September 23, 2016
Author(s)
Cherno Jaye, Tobias Weidner, J. E. Baio, A. P. Hitchcock, Daniel A. Fischer
It is shown that the self-assembly of diamagnetic molecule sub-monolayers on a surface can be influenced by magnetic stray field landscapes emerging from artificially fabricated magnetic domains and domain walls. The directed local chemisorption of

Microcalorimeter Spectroscopy at High Pulse Rates: a Multi-Pulse Fitting Technique

August 24, 2015
Author(s)
Joseph W. Fowler, Bradley K. Alpert, William B. Doriese, Young Il Joe, Galen C. O'Neil, Cherno Jaye, Joel N. Ullom, Daniel A. Fischer, Daniel S. Swetz
Transition edge sensor microcalorimeters can measure x-ray and gamma-ray energies with very high energy resolution and high photon-collection efficiency. For this technology to reach its full potential in future x-ray observatories, each sensor must be

Dry graphene transfer print to polystyrene and ultra-high molecular weight polyethylene ? detailed chemical, structural, morphological and electrical characterization

May 17, 2015
Author(s)
Evegeniya Lock, Dean DeLongchamp, Scott Schmucker, Blake Simpkins, Matthew Laskoski, Shawn Mulvaney, Daniel R. Hines, Mira Baraket, Sandra Hernandez, Jeremy Robinson, Paul Sheehan, Cherno Jaye, Daniel A. Fischer, Scott Walton
In this paper we apply a transfer print approach that relies on differential adhesion to remove graphene from Cu foil to polystyrene (PS) and ultra-high molecular weight polyethylene (UHMW PE) without etching of the metal foil. The polymer surfaces are

High-resolution X-ray emission spectroscopy with transition-edge sensors: present performance and future potential

May 1, 2015
Author(s)
W.Bertrand (Randy) Doriese, Joseph Fowler, Daniel Swetz, Cherno Jaye, Daniel A. Fischer, Carl D. Reintsema, Douglas Bennett, Leila R. Vale, Gene C. Hilton, Dan Schmidt, Joel Ullom, Jens Uhlig, Ujjwal Mandal, Galen O'Neil, Luis Miaja Avila, Young I. Joe, wilfrid fullagar, Fredrick P. Gustafsson, Dharma Kurunthu, Villy Sundstrom
X-ray emission spectroscopy (XES) is a powerful element-selective tool to analyze the oxidation states of atoms in complex compounds, determine their electronic configuration, and identify unknown compounds in challenging environments. Until now the low

Interrogating the Carbon and Oxygen K-edge NEXAFS of a CO2-dosed Hyperbranched Aminosilica

December 19, 2014
Author(s)
Laura Espinal, Martin L. Green, Dean M. DeLongchamp, Watcharop Chaikittisilp, Jarod C. Horn, Miles Sakwa-Novak, Cherno Jaye, Daniel A. Fischer, Nicholas Brunelli, Christopher Jones
Near edge x-ray absorption fine structure (NEXAFS) spectroscopy was used to study the adsorption of CO2 in a hyperbranched aminosilica (HAS) compound, a porous solid state material with great potential for carbon capture applications. After dosing a

Interfacial Mechanical Properties of n-Alkylsilane Monolayers on Silicon Substrates

February 1, 2013
Author(s)
Brian G. Bush, Frank W. DelRio, Cherno Jaye, Daniel A. Fischer, Robert F. Cook
The interfacial properties of n-alkylsilane self-assembled monolayers on silicon were investigated by normal force spectroscopy and lateral force measurements and correlated with molecular structure via near-edge X-ray absorption fine structure (NEXAFS)

ELECTRICAL AND PHYSICAL CHARACTERIZATION OF BILAYER CARBOXYLIC ACID FUNCTIONALIZED MOLECULAR LAYERS

January 30, 2013
Author(s)
Sujitra J. Pookpanratana, Joseph W. Robertson, Cherno Jaye, Daniel A. Fischer, Curt A. Richter, Christina A. Hacker
We have used Flip Chip Lamination (FCL) to form monolayer and bilayer molecular junctions of carboxylic acid-containing molecules with Cu atom incorporation. Carboxylic acid-terminated monolayers are self-assembled onto ultrasmooth Au using thiol chemistry

Molecular beam growth of graphene nanocrystals on dielectric substrates

November 27, 2012
Author(s)
Daniel A. Fischer, Ulrich Wurstbauer, Theanne Schiros, Cherno Jaye, A. S. Plaut, R. He, Albert Rigosi, Liuyan Zhao, Christopher Gutierrez, P. Kim, L. N. Pfeiffer, A. Pasupathy, A. Pinczuk, J. M. Garcia
A variety of methods have been reported to create graphene. These include the pervasive mechanical exfoliation of graphite1, as well as methods that obtain large area graphene such as thermal decomposition of SiC2,3, chemical vapor deposition on transition

Molecular Order in High-Efficiency Polymer/Fullerene Bulk Heterojunction Solar Cells

September 22, 2011
Author(s)
Matthew R. Hammond, Regis J. Kline, Andrew A. Herzing, Lee J. Richter, David Germack, Hyun W. Ro, Christopher L. Soles, Daniel A. Fischer, Tao Xu, Luping Yu, Michael F. Toney, Dean M. DeLongchamp
We report quantitative measurements of ordering, molecular orientation, and nanoscale morphology in the active layer of bulk heterojunction organic photovoltaic cells based on a thieno[3,4-b]thiophene-alt-benzodithiophene copolymer (PTB7), which has been

Structure-property relationships for methyl-terminated alkyl self-assembled monolayers

July 20, 2011
Author(s)
Frank W. DelRio, Dave Rampulla, Cherno Jaye, Gheorghe Stan, Richard S. Gates, Daniel A. Fischer, Robert F. Cook
Structure-property relationships for methyl-terminated alkyl self-assembled monolayers (SAMs) are developed using near-edge X-ray absorption fine structure spectroscopy (NEXAFS) and atomic force microscopy (AFM). NEXAFS C K-edge spectra are used to compute

Characterization of the non-uniform reaction in chemically-amplified calix[4]resorcinarene molecular resist thin films

July 19, 2011
Author(s)
Vivek M. Prabhu, Shuhui Kang, Regis J. Kline, Dean M. DeLongchamp, Daniel A. Fischer, Wen-Li Wu, Sushil K. Satija, Jing Sha, Christopher K. Ober, Peter V. Bonnesen
The ccc stereoisomer-purified tert-butoxycarbonyloxy (t-Boc) protected calix[4]resorcinarene molecular resists blended with photoacid generator exhibit a non-uniform photoacid catalyzed reaction in thin films. The surface displays a reduced reaction extent

Influence of substrate on crystallization in polythiophene/fullerene blends

January 13, 2011
Author(s)
Lee J. Richter, Christine He, David Germack, R Joseph Kline, Dean DeLongchamp, Daniel A. Fischer, Chad R. Snyder, James G. Kushmerick
The nanoscale morphology of the active layer in organic, bulk heterojunction (BHJ) solar cells is crucial to device performance. Often a combination of casting conditions and post deposition thermal treatment are used to optimize the morphology. In general

Enhanced Water Splitting Performance of Potassium-Adsorbed Titania Nanotube Arrays

December 7, 2009
Author(s)
Christiaan Richter, Cherno Jaye, Eugen Panaitescu, Daniel A. Fischer, Laura H. Lewis, Ronald J. Willey, Latika Menon
It is demonstrated that vertically-aligned titania nanotube planar arrays fabricated by electrochemical anodization using standard potassium-containing electrolytes invariably contain a significant amount of surface-adsorbed potassium ions that enhance the