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Physics

Spectroscopy

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Displaying 1 - 25 of 1697

High-Stability Single-Ion Clock with 5.5 x 10^-19 Systematic Uncertainty

April 21, 2025
Author(s)
Mason Marshall, Daniel Rodriguez Castillo, Willa Dworschack, Alexander Aeppli, Kyungtae Kim, Dahyeon Lee, William Warfield, Nicholas Nardelli, Tara Fortier, Jun Ye, David Ray Leibrandt, David Hume
We report a single-ion optical atomic clock with fractional frequency uncertainty of 5.5 x 10^-19 and frequency stability of 3.5 x 10^-16/sqrttau/s}, based on quantum logic spectroscopy of a single 27Al+ ion. A co-trapped 25Mg+ ion provides sympathetic

Compact Blackbody Radiation Atomic Sensor: Measuring Temperature using Optically Excited Atoms in Vapor Cells

April 17, 2025
Author(s)
David La Mantia, Mingxin Lei, Nikunjkumar Prajapati, Noah Schlossberger, Matthew Simons, Christopher Holloway, Julia Scherschligt, Stephen Eckel, Eric Norrgard
We demonstrate a blackbody radiation thermometer based on optically excited rubidium atoms in a vapor cell. Operating as a calibrated contact thermometer from 308K to 343 K, we realize temperature uncertainty as low as 0.04 %, and statistical temperature

Contributions of argon, nitrogen, and oxygen to air broadening in the oxygen A-band

April 16, 2025
Author(s)
Leah Stevenson, Mitchio Okumura, Joseph Hodges, Erin Adkins
The oxygen (O2) A-band is used to determine the air mass in ground- and space-based remote sensing measurements because the O2 mixing ratio in Earth's atmosphere is constant. Because errors in the retrieved air mass propagate to measurements of target gas

Efficient Energy Transfer and Photoluminescence Enhancement in 2D MoS2/bulk InSe van der Waals Heterostructures

April 13, 2025
Author(s)
Michael Altvater, Christopher Stevens, Nicholas Pike, Joshua Hendrickson, Rahul Rao, Sergiy Krylyuk, Albert Davydov, Deep Jariwala, Ruth Patcher, Michael Snure, Nicholas Glavin
Heterostructures between 2D and 3D electron systems remain critically important in developing novel and efficient optoelectronic and electronic devices. In this study, a vertical heterojunction between monolayer MoS2 and bulk InSe was developed. This

New beyond-Voigt line-shape pro le recommended for the HITRAN database

March 27, 2025
Author(s)
Piotr Wcislo, N. Stolarczyk, M. Slowinski, H. Jozwiak, Daniel Lisak, R. Ciurylo, A. Cygan, F. Schreier, C.D. Boone, A. Castrillo, L. Gianfrani, Y. Tan, S-M. Hu, Erin Adkins, Joseph Hodges, H. Tran, H.N. Ngo, J.M- Hartmann, A. Campargue, S. Beguier, R.J. Hargreaves, L.S. Rothman, I.E. Gordon
Parameters associated with the collisional perturbation of spectral lines are essential for modeling the absorption of electromagnetic radiation in planetary atmospheres. The HITRAN molecular spectroscopic database provides these parameters, although

A low-cost ultrasonic absorption spectrometer mainly using off-the-shelf parts

March 11, 2025
Author(s)
Michelle Crouse, Malgorzata Musial, Jason Widegren, Jacob Pawlik, Bryan Bosworth, Nathan Orloff, Aaron Hagerstrom, Angela Stelson, Robert Lirette
Ultrasonic absorption spectroscopy can probe intermolecular interactions that inform research into chemical engineering and pharmaceutical manufacturing processes. The only commercial ultrasonic spectrometer costs over one hundred thousand dollars, putting

An Accurate Determination of O2 A-band Line Intensities through Experiment and Theory

February 27, 2025
Author(s)
Erin Adkins, Sergei Yurchenko, Wilfrid Somogyi, Joseph Hodges
Accurate intensities of the O2 A-band 〖[b〗^1 Σ_g^+⟵X^3 Σ_g^- (0,0)] centered about 760 nm are essential to reduce biases in satellite- and ground-based remote measurements of column-integrated air mass and greenhouse gas concentration. In support of these

Quantum Emitters Induced by High Pressure and UV Laser Irradiation in Multilayer GaSe

February 14, 2025
Author(s)
Sinto Varghese, Sichenge Wang, Bimal Neupane, Bhojraj Bhandari, Yan Jiang, Roberto Gonzalez Rodriguez, Sergiy Krylyuk, Albert Davydov, Hao Yan, Yuanxi Wang, Anupama Kaul, Jingbiao Cui, Yuankun Lin
In this work, we report on defect generation in multilayer GaSe through hydrostatic pressure quenching and UV laser irradiation. The Raman line width from the UV 266 nm irradiated sample is much wider than that in pressure-quenched GaSe, corresponding to a

Application of hard x-ray and gamma-ray TES microcalorimeters at an accelerator facility

January 24, 2025
Author(s)
Takeshi Saito, Shinji Okada, Yuichi Toyoma, Toshiyuki Azuma, Goncalo Baptista, Daniel Becker, Douglas Bennett, William Doriese, Joseph Fowler, Johnathon Gard, Tadashi Hashimoto, Ryota Hayakawa, Tasuku HAYASHI, Yuto Ichinohe, Josef Imrek, Paul Indelicato, Tadaaki Isobe, Sohtaro Kanda, Naritoshi Kawamura, John Mates, Yasuhiro Miyake, Kelsey Morgan, Hirofumi Noda, Galen O'Neil, Takuma Okumura, Nancy Paul, Daniel Schmidt, Kouichiro Shimomura, Patrick Strasser, Daniel Swetz, Tadayuki Takahashi, Motonobu Tampo, Joel Ullom, Izumi Umegaki, Joel Weber, Shinya Yamada, Daikang Yan
The x-ray spectroscopy of the muonic atom has attracted atomic, nuclear, and particle physicists since its discovery. The properties of a muonic atom, such as its binding energy or atomic radius, are different from an ordinary atom because of the

International Comparison CCQM-P229: Pilot Study to Measure Absolute Line Intensities of Selected 12C16O Transitions

January 24, 2025
Author(s)
Joseph Hodges, Zachary Reed, Katarzyna Bielska, Manfred Birk, Ruimin Guo, Gang Li, Jeong Sik Lim, Daniel Lisak, Georg Wagner
We present primary spectroscopic measurements of line intensities in the 3-0 vibrational band of 12C16O. This international measurement campaign was organized under the auspices of the Consultative Committee for Amount of Substance (CCQM) and involved six

Platinum Hydride Formation during Cathodic Corrosion in Aqueous Solutions

January 22, 2025
Author(s)
Thomas Hersbach, Angel T. Garcia-Esparza, Selwyn Hanselman, Thijs Hoogenboom, Ian McCrum, Dimitra Anastasiadou, Jeremey Feaster, Thomas Jaramillo, John Vinson, Thomas Kroll, Amanda Garcia, Petr Krtil, Dimosthenis Sokaras, Marc Koper
Cathodic corrosion is an electrochemical phenomenon that dramatically etches metals under commonly used electrocatalytic conditions. Though cathodic corrosion is thought to occur by forming a metal-containing anion, such an ion has not yet been observed

Towards Precision Spectroscopy of Antiprotonic Atoms for Probing Strong-field QED

January 15, 2025
Author(s)
Goncalo Baptista, Shikha Rathi, Michael Roosa, Quentin Senetaire, Jonas Sommerfeldt, Toshiyuki Azuma, Daniel Becker, Francois Butin, Ofir Eizenberg, Joseph Fowler, Hiroyuki Fujioka, Davide Gamba, Nabil Garroum, Mauro Guerra, Tadashi Hashimoto, Takashi Higuchi, Paul Indelicato, Jorge Machado, Kelsey Morgan, Francois Nez, Jason Nobles, Ben Ohayon, Shinji Okada, Daniel Schmidt, Daniel Swetz, Joel Ullom, Pauline Yzombard, Marco Zito, Nancy Paul
PAX (antiProtonic Atom X-ray spectroscopy) is a new experiment with the aim to test strong-field quantum electrodynamics (QED) effects by performing high-precision x-ray spectroscopy of antiprotonic atoms. By utilizing advanced microcalorimeter detection

Glass microwave microfluidic devices for broadband characterization of diverse fluids

November 15, 2024
Author(s)
Jacob Pawlik, Tomasz Karpisz, Yasaman Kazemipour, Nicholas Derimow, Sarah Evans, Bryan Bosworth, Christian Long, Nathan Orloff, James Booth, Angela Stelson
We demonstrate a glass microwave microfluidic device for determining the permittivity of a wide range of liquid chemicals from 100 MHz to 10 GHz with relatively low uncertainty. Conventional microwave microfluidic devices use polymer-based microfluidic

Spectroscopy of photoionization from the 1E singlet state in nitrogen-vacancy centers in diamond

October 17, 2024
Author(s)
Sean Blakley, Thuc Mai, Stephen Moxim, Jason Ryan, Adam Biacchi, Angela Hight Walker, Robert McMichael
The 1E—1A1 singlet manifold of the negatively charged nitrogen vacancy (NV −) center in diamond plays a central role in the quantum information and quantum sensing applications of the NV − center. However, the energy of this manifold within the diamond

Unusually strong near-infrared photoluminescence of highly transparent bulk InSe flakes

September 23, 2024
Author(s)
Jamie Geng, Dehui Zhang, Inha Kim, Hyong Min Kim, Naoiki Higashitarumizu, I K M Reaz Rahman, Lam Lam, Joel W. Ager III, Albert Davydov, Sergiy Krylyuk, Ali Javey
Bulk γ-InSe has a direct bandgap of 1.24 eV, which corresponds to near infrared wavelengths (λ = 1.0 µm) useful in optoelectronic applications from biometric detectors to silicon photonics. However, its potential for optoelectronic applications is largely
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