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Materials

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Displaying 826 - 850 of 2328

TOPOLOGY OF VOIDS AND CHANNELS IN SELECTED PORPHYRINIC COMPOUNDS

December 1, 2019
Author(s)
Lawrence P. Cook, Greg Brewer, Daniel Siderius, Winnie Wong-Ng
Porphyrinic compounds are of increasing interest to the materials science community, yet little attention has been paid to crystallographically controlled voids and channels in these materials. We have conducted an initial survey of the voids and channels

Exploring the Limits of Bottom-Up Gold Filling to Fabricate Diffraction Gratings

November 27, 2019
Author(s)
Daniel Josell, Stephen J. Ambrozik, Maureen E. Williams, A E. Hollowell, Christian Arrington, Shinichiro Muramoto, Thomas P. Moffat
Gold deposition on rotating disk electrodes, Bi3+ adsorption on planar Au films and superconformal Au filling of trenches up to 45 m deep are examined in Bi+3-containing Na3Au(SO3)2 electrolytes with pH between 9.5 and 11.5. Higher pH is found to increase

Unexpectedly Strong Size-Sieving Ability in Carbonized Polybenzimidazole for Membrane H2/CO2 Separation

November 21, 2019
Author(s)
Maryam Omidvar, Hien Nguyen, Liang Huang, Cara Doherty, Anita Hill, Christopher Stafford, Xianshe Feng, Mark Swihart, Haiqing Lin
Polymers with high permeability and strong size-sieving ability are needed for H2/CO2 separation at temperatures ranging from 100 °C to 300 °C to enable an energy-efficient pre- combustion CO2 capture process. However, such polymers usually suffer from a

Damping Enhancement in Coherent Ferrite-Insulating-Paramagnet Bilayers

November 19, 2019
Author(s)
Jacob J. Wisser, Alexander Grutter, Dustin A. Gilbert, Alpha T. N'Diaye, Christoph Klewe, Padraic Shafer, Elke Arenholz, Yuri Suzuki, Satoru Emori
High-quality epitaxial ferrites, such as low-damping MgAl-ferrite (MAFO), are promising nanosclae building blocks for all-oxide heterostructures driven by pure spin current. However, the impact of oxide interfaces on spin dynamics in such heterostructures

Dynamic Equivalence between Soft Star Polymers and Hard Spheres

November 19, 2019
Author(s)
Zhe Wang, Antonio Faraone, Panchao Yin, Lionel Porcar, Yun Liu, Changwoo Do, Kunlun Hong, Wei-Ren Chen
We measure a series of star polymer dispersions to study the dynamics of soft colloidal liquids. We find that as the concentration increases, the slowing of the long-time self-diffusivity of the star polymer, normalized by the short-time self-diffusivity

Chalcogenide Topological Insulators

November 15, 2019
Author(s)
Joseph A. Hagmann
The purpose of this chapter is to introduce the reader to the chalcogenide materials systems that host the topological insulator phase of quantum matter. Specifically, the HgTe quantum well 2D topological insulator system and the V2VI3-type bismuth- and

Enhanced Gas Uptake in a Microporous Metal-Organic Framework via a Sorbate Induced-Fit Mechanism

November 13, 2019
Author(s)
Mei-Hui Yu, Brian Space, Douglas Franz, Wei Zhou, Chaohui He, Libo Li, Rajamani Krishna, Ze Chang, Wei Li, Tong-Liang Hu, Xian-He Bu
Physical adsorption of gas molecules in microporous materials is an exothermic process, with desorption entropy driving a decrease in uptake with temperature. Enhanced gas sorption with increasing temperature is rare in porous materials and is indicative

Tailoring the Pore Geometry and Chemistry in Microporous Metal-Organic Frameworks for High Methane Storage Working Capacity

November 13, 2019
Author(s)
Kai Shao, Jiyan Pei, Jia-Xin Wang, Yu Yang, Yuanjing Cui, Wei Zhou, Taner N. Yildirim, Bin Li, Banglin Chen, Guodong Qian
We realize that tailoring pore size/geometry and Chemistry, by virture of alkynl or naphthalene replacing phenyl within a series of isomorphic MOFs, can optimize methane storage working capacities, affording an exceptionally high working capacity of 203 cm

Recent trends in crystallography a current IUCr journals perspective

November 1, 2019
Author(s)
Andrew J. Allen
The International Union of Crystallography (IUCr) publishes papers in nine scientific journals, including its high-impact, cross-cutting open-access journal, IUCrJ, plus its data publication, IUCrData. Where are these papers cited? To what degree are

Reversible Epitaxial Electrodeposition of Metals in Battery Anodes

November 1, 2019
Author(s)
Jingxu Zheng, Qing Zhao, Tian Tang, Jiefu Yin, Calvin D. Quilty, Genesis D. Renderos, Xiaotun Liu, Yue Deng, Lei Wang, David C. Bock, Cherno Jaye, Esther S. Takeuchi, Kenneth J. Takeuchi, Amy C. Marschilok, Lynden A. Archer
The propensity of metals to form irregular and non-planar electrodeposits at liquid/solid interfaces has emerged as a fundamental barrier to high-energy, rechargeable batteries that utilize metal anodes. We report an epitaxial mechanism to regulate

Effect of Flexibility and Nanotriboelectrification on the Dynamic Reversibility of Water Intrusion into Nanopores: Pressure-Transmitting Fluid with Frequency-Depending Dissipation Capability

October 30, 2019
Author(s)
Alexander Lowe, Nikolay Tsyrin, Miroslaw Chorazewski, Pawel Zajdel, Michal Mierzwa, Juscelino Leao, Markus Bleuel, Tong Feng, Dong Luo, Mian Li, Dan Li, Victor Stoudenets, Sebastian Pawlus, Abdessamad Faik, Yaroslav Grosu
In this work the effect of a porous material´s flexibility on the dynamic reversibility of a non-wetting liquid intrusion was explored experimentally. For this purpose, high-pressure water intrusion together with high-pressure in-situ small angle neutron

Tunable Magnetic Ordering through Cation Selection in Entropic Spinel Oxides

October 21, 2019
Author(s)
Brianna Musico, Quinton Wright, T. Zac Ward, Alexander Grutter, Elke Arenholz, Dustin Gilbert, David Mandrus, Veerle Keppens
Twelve multicomponent spinels, comprised of (Mg, Cr, Mn, Co, Fe, Ni, Cu, and/or Zn)(Cr, Fe or Al) 2O 4, were prepared using solid state synthesis methods, resulting in nine homogenous, single phase samples with a Fm-3m structure, and three samples with

Orientational Distribution Function of Aligned Elongated Molecules and Particulates Determined from Their Scattering Signature

October 15, 2019
Author(s)
Guan-Rong Huang, Yangyang Wang, Changwoo Do, Yuya Shinohara, Takeshi Egami, Lionel Porcar, Yun Liu, Wei-Ren Chen
We present a strategy for quantitatively evaluating the field-induced alignment of non-spherical particles using small angle scattering techniques. The orientational distribution function (ODF) is determined from the anisotropic scattering intensity via

Biomimetic Approach to Inhibition of Photooxidation in Organic Solar Cells Using Beta-Carotene as an Additive

October 14, 2019
Author(s)
Sebastian Engmann, Vida Turkovic, Michela Prete, Mikkel Bregnhoj, Liana Inasaridze, Dmytro Volyniuk, Filipp Obrezkov, Juozas V. Grazulevicius, Horst G. Rubahn, Pavel Troshin, Peter R. Ogilby, M. Madsen
Recent improvements in the power conversion efficiencies of organic photovoltaic (OPV) cells have highlighted the fact that OPV device lifetimes are now the main bottleneck for further advances of this technology. As such, understanding and controlling

Chain and Ion Dynamics in Precise Polyethylene Ionomers

October 11, 2019
Author(s)
Christopher L. Soles, Amalie Frischknecht, Benjamin Paren, Robert Middleton, Karen Winey, Jason Koski, Madhu Sudan Tyagi, Jacob Daniel Tarver
We analyze the dynamics from microsecond-long, atomistic molecular dynamics (MD) simulations of a series of precise poly(ethylene-co-acrylic acid) ionomers neutralized with lithium, with three different spacer lengths between acid groups on the ionomers

Observation of Strong Polarization Enhancement in Ferroelectric Tunnel Junctions

October 9, 2019
Author(s)
Linze Li, Xiaoxing Cheng, Thomas Blum, Huaixun Huyan, Yi Zhang, Colin A. Heikes, Xingxu Yan, Chaitanya Gadre, Toshihiro Aoki, Mingjie Xu, Lin Xie, Zijian Hong, Carolina Adamo, Darrell G. Schlom, Long-Qing Chen, Xiaoqing Pan
Ferroelectric heterostructures, with capability of storing data at ultrahigh densities, could act as the platform for next-generation memories. The development of new device paradigms has been hampered by the long-standing notion of inevitable

Lattice theory for binding of linear polymers to a solid substrate from polymer melts: II. Influence of van der Waals interactions and chain semi?exibility on molecular binding and adsorption

September 30, 2019
Author(s)
Jack F. Douglas, Jacek Dudowicz, Karl Freed
The Polymeric Langmuir Theory (PLT), developed in Paper I, is employed to investigate the influence of van der Waals interactions and chain rigidity on the thermodynamics of the reversible molecular binding to interfaces in one component polymer fluids
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