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Materials

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Displaying 801 - 825 of 2343

Field Ion Emission in an Atom Probe Microscope Triggered by Femtosecond-Pulsed Coherent Extreme Ultraviolet Light

March 12, 2020
Author(s)
Ann C. Chiaramonti Debay, Luis Miaja Avila, Benjamin W. Caplins, Paul T. Blanchard, Norman A. Sanford, Brian Gorman, David R. Diercks
This paper reports construction of an extreme ultraviolet (EUV) radiation-triggered atom probe tomograph and describes the results from initial experiments on amorphous SiO2. Femtosecond-pulsed coherent EUV radiation of 29.6 nm wavelength (41.85 eV photon

Nanoscale Pattern Decay Monitored via in-situ Heated Atomic Force Microscopy

March 12, 2020
Author(s)
Sonal Bhadauriya, Jianan Zhang, Jaejun Lee, Michael R. Bockstaller, Alamgir Karim, Richard J. Sheridan, Christopher Stafford
We combine in-situ heated atomic force microscopy (AFM) with automated line-by-line spectral analysis to quantify the relaxation or decay of nanopatterned polymer films at temperatures above the glass transition. This approach enables assessment of pattern

Large Enhancement of Magnetocaloric and Barocaloric Effects by Hydrostatic Pressure in La(Fe 0.92 Co 0.08 ) 11.9 Si 1.1 with a NaZn 13 -Type Structure

March 10, 2020
Author(s)
Jiazheng Hao, Fengxia Hu, Jian-Tao Wang, Fei-Ran Shen, Zibing Yu, Houbo Zhou, Hui Wu, Qingzhen Huang, Kaiming Qiao, Jing Wang, Jun He, Lunhua He, Ji-Rong Sun, Baogen Shen
Solid state refrigeration based on caloric effect has been regarded as an attractive alternative to conventional gas compression technique. Boosting the caloric effect of a system to its optimum is a long-term pursuit. Here, we report enhanced

Hydrodynamic Factors Influencing Mineral Dissolution Rates

March 9, 2020
Author(s)
Nicos Martys, Jeffrey W. Bullard, Pan Feng, Shaoxiong Ye
Solution flow profiles near a mineral surface can have significant influences on the local thermodynamic driving force and, potentially, the rate-controlling kinetic mechanism of its dissolution or precipitation. These influences are investigated here both

Strain-Induced Majority Carrier Inversion in Ferromagnetic Epitaxial LaCoO^d3-d Thin Films

March 4, 2020
Author(s)
Vipul Chaturvedi, Jeff Walter, Arpita Paul, Alexander Grutter, Brian Kirby, Jong Seok Jeong, Hua Zhou, Zhan Zhang, Biqiong Yu, Martin Greven, K. Andre Mkhoyan, Turan Birol, Chris Leighton
Tensile-strained LaCoO 3-δ thin films are ferromagnetic, in sharp contrast to the zero-spin bulk, although no clear consensus has emerged as to the origin of this phenomenon. While magnetism has been heavily studied, relatively little attention has been

Cone-Spiral Magnetic Ordering Dominated Lattice Distortion and Giant Negative Thermal Expansion in Fe-Doped MnNiGe Compounds

March 1, 2020
Author(s)
Feiran Shen, Houbo Zhou, Fengxia Hu, Jian-Tao Wang, Sihao Deng, Baotian Wang, Hui Wu, Qingzhen Huang, Jing Wang, Jie Chen, Lunhua He, Jiazheng Hao, Zibing Yu, Feixiang Liang, Tianjiao Liang, Jirong Sun, Baogen Shen
Negative thermal expansion (NTE) has emerged as one of intense research topics to meet the demands of precision industry for compensating positive thermal expansion (PTE) properties. The adjustment of NTE behavior is the key for tailoring thermal expansion

Perovskite-Related ReO 3 -Type Structures

March 1, 2020
Author(s)
Hayden A Evans, Yue Wu, Ram Seshadri, Anthony K. Cheetham
ReO 3-type structures can be described as ABX 3 perovskites in which the A-cation site is unoccupied. They therefore have the general composition BX 3, where B is normally a cation and X is a bridging anion. The chemical diversity of such structures is

Enhanced Dynamics of Confined Polymers near the Immiscible Polymer-Polymer Interface: Neutron Reflectivity Studies

February 18, 2020
Author(s)
Kyoung-Il Jo, Younghoon Oh, Bong June Sung, Tae-Ho Kim, Min Seop Um, Woo Jin Choi, Joona Bang, Guangcui Yuan, Sushil K. Satija, Jaseung Koo
For polymer-blend films, local dynamics in confined polymer domains tend to differ from the bulk due to significant contributions from the polymer-polymer interface. Herein, we investigated the diffusion dynamics of entangled polymer thin films confined

Metal adsorbate interactions and the convergence of density functional calculations

February 10, 2020
Author(s)
Christoph Rohmann, Maicol A. Ochoa, Michael P. Zwolak
The adsorption of metal atoms on nanostructures, such as graphene and nanotubes, plays an important role in catalysis, electronic doping, and tuning material properties. Quantum chemical calculations permit the investigation of this process to discover

Dynamic Arrest of Adhesive Hard Rod Dispersions

February 7, 2020
Author(s)
Ryan P Murphy, Harold Wickes Hatch, Nathan NMN Mahynski, Vincent K. Shen, Norman J. Wagner
Dynamic arrest transitions of model, thermoreversible dispersions of adhesive hard rods are measured as a function of absolute temperature Τ = 15 -40 °C, aspect ration L/D{approximately equal}3-7, and volume fraction φ0.1-0.5. The critical gel temperature

Dynamic Heterogeneity and Collective Motion in Star Polymer Melts

February 4, 2020
Author(s)
Jack F. Douglas, Jinpeng Fan, Hamed Emamy, Francis W. Starr, Alexandros Chremos
While glass formation of linear chain polymers has been widely explored, comparatively little is known about glass formation in star polymer melts. We study the segmental dynamics of star polymers via molecular dynamics simulations and contrast the

Alignment of Worm-like Micelles at Intermediate and High Shear Rates

February 1, 2020
Author(s)
Brisa Arenas-Gomez, Cristina Garza, Yun Liu, Rolando Castillo
Hypothesis. Rheology combined with Small Angle Neutron Scattering (Rheo-SANS) can determine the local structural order in Worm-like Micelle (WLM) solutions, when the shear rate increases beyond the ending of the gradient shear banding, where the micellar

Emergent Electric Field Control of Phase Transformation in Oxide Superlattices

February 1, 2020
Author(s)
Di Yi, Yujia Wang, Olaf M. J. van t'Erve, Liubin Xu, Hongtao Yuan, Michael J. Veit, Purnima P. Balakrishnan, Yongseong Choi, Alpha T. N'Diaye, Padraic Shafer, E. Arenholz, Alexander Grutter, Haixuan Xu, Pu Yu, Berend T. Jonker, Yuri Suzuki
Electric fields have been shown to transform materials with respect to their structure and properties, thus enabling many applications ranging from batteries to spintronics. Recently electrolytic gating, which can generate large electric fields and voltage

Pressure-Thresholded Response in Cylindrically Shocked Cyclotrimethylene Trinitramine (RDX)

February 1, 2020
Author(s)
Leora E. Dresselhaus-Cooper, Dmitro Martynowych, Fan Zhang, Charlene Tsay, Jan Ilavsky, SuYin Wang, Yu-Sheng Chen, Lara Leininger, Keith A. Nelson
We demonstrate a strongly thresholded response in cyclotrimethylene trinitramine (RDX) that is cylindrically shocked using a novel waveguide geometry. Using ultrafast single-shot multi-frame imaging, we demonstrate that a 100-μm diameter single crystal of

Reversed Ethane/Ethylene Adsorption in Metal-Organic Frameworks via Introduction of Oxygen

February 1, 2020
Author(s)
Ling Yang, Wei Zhou, Hao Li, Ali Alsalme, Litao Jia, Jinping Li, Libo Li, Banglin Chen
Separation of ethane from ethylene is a very important but challenging process in the petrochemical industry. Finding an alternative method would reduce the energy needed to make the 170 million tons of ethylene manufactured worldwide each year. Adsorptive
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