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Physics

Spectroscopy

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Displaying 51 - 75 of 907

Zeeman effect in the weak and intermediate field regime of Kr isotopes at the linear plasma device PSI-2

February 16, 2024
Author(s)
Yuri Ralchenko, DIPTI DIPTI, Oleksandr Marchuk, Marc Sackers, Stephan Ertmer, Sebastijan Brezinsek, Arkadi Kreter
Laser absorption spectroscopy provides high-resolution spectra of atomic transitions that reveal many often inaccessible nuances. Correctly analyzing the absorption spectra is impossible without accurately capturing the line shape. We demonstrate in this

Multi-code Benchmark on Ti K-edge X-ray Absorption Spectra of Ti-O Compounds

January 11, 2024
Author(s)
Fanchen Meng, Benedikt Maurer, Fabian Peschel, Sencer Selcuk, Xiaohui Qu, Mark S Hybertsen, Christian Vorwerk, Claudia Draxl, John Vinson, Deyu Lu
X-ray absorption spectroscopy (XAS) is an element-specific materials characterization technique that is sensitive to structural and electronic properties. First-principles simulated XAS has been widely used as a powerful tool to interpret experimental

Tracking Active Phase Behavior on Boron Nitride during the Oxidative Dehydrogenation of Propane Using Operando X-Ray Raman Spectroscopy

November 6, 2023
Author(s)
Melissa Cendejas, Oscar Paredes Mellone, Unni Kurumbail, Zisheng Zhang, Jacob Jansen, Faysal Ibrahim, Son Dong, John Vinson, Anastassia Alexandrova, Dimosthenis Sokaras, Simon Bare, Ive Hermans
Hexagonal boron nitride (hBN) is a highly selective catalyst for the oxidative dehydrogenation of propane (ODHP) to propylene. Using a variety of ex situ characterization techniques, the activity of the catalyst has been attributed to the formation of an

Nanosecond time-resolved dual-comb absorption spectroscopy

October 30, 2023
Author(s)
David Long, Matthew Cich, Carl Mathurin, Garrett Mathews, Adam Heiniger, Augustine Frymire, Gregory Rieker
Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. Although there have been tremendous strides in direct frequency comb

Single-Detector Double-Beam Modulation for High-Sensitivity Infrared Spectroscopy

October 25, 2023
Author(s)
Seongmin Kim, Yow-Ren Chang, Young Jong Lee
Balanced detection based on double beams is widely used to reduce common-mode noises, such as laser intensity fluctuation and irregular wavelength scanning, in absorption spectroscopy. However, employing an additional detector can increase the total system

Next-Generation Chip-Scale Atomic Clocks

October 16, 2023
Author(s)
John Kitching, Matthew Hummon, William McGehee, Ying-Ju Wang, Susan Schima
We describe work toward the development of next-generation chip-scale atomic clocks, which combine small size, low power consumption and manufacturability with high frequency stability. The use of optical transitions in microfabricated vapor cells improves

Strain-activated stimulated emission from multilayer MoSe2 in a narrow operation window

September 24, 2023
Author(s)
Yuankun Lin, Noah Hurley, Steve Kamau, Evan Hathaway, Yan Jiang, Roberto Gonzalez Rodriguez, Sinto Varghese, Sergiy Krylyuk, Albert Davydov, Yuanxi Wang, Anupama Kaul, Jingbiao Cui
Herein, photoluminescence (PL) and fluorescence lifetime imaging (FLIM) in multilayer MoSe2 are studied. Strain-activated stimulated emission via defect levels in multilayer MoSe2 under laser excitation is observed, for the first time in defects of

Open-path measurement of stable water isotopologues using mid-infrared dual-comb spectroscopy

September 8, 2023
Author(s)
Daniel Herman, Griffin Mead, Fabrizio Giorgetta, Esther Baumann, Nathan Malarich, Brian Washburn, Nathan R. Newbury, Ian Coddington, Kevin Cossel
We present an open-path mid-infrared dual-comb spectrometer (DCS) capable of precise measurement of the stable water isotopologues H216O and HD16O. This system runs in a remote configuration at a rural test site with high uptime and achieves a precision of

Radiative Decay Rate and Branching Fractions of MgF

September 8, 2023
Author(s)
Eric Norrgard, Catherine Cooksey, Stephen Eckel, Nickolas Pilgram, Kayla Rodriguez, Howard W. Yoon, Yuly Andrea Chamorro Mena, Lukas Pasteka, Anastasia Borschevsky
Here we report measured and calculated values of radiative decay rates and vibrational branching fractions for the A$^2\Pi$ state of MgF. The decay rate measurements use time-correlated single photon counting with roughly 1\,\% total uncertainty. Branching

Dual-Comb Spectroscopy of Carbon Dioxide and Methane Across a 14.5 km Long Outdoor Path

September 1, 2023
Author(s)
Fabrizio Giorgetta, Esther Baumann, Brian Washburn, Nathan Malarich, Jean-Daniel Deschenes, Ian Coddington, Nathan Newbury, Kevin Cossel
Greenhouse-gas dual-comb spectroscopy is extended to a city-scale 14.5-km path length using remote receiver and data acquisition. This configuration enables lower link losses and longer path lengths compared to folded paths with a remote retroreflector

Structural Origin of Recovered Ferroelectricity in BaTiO3 Nanoparticles

August 24, 2023
Author(s)
Bruce D. Ravel, Trevor Tyson, Han Zhang, Sizhan Liu, SANJIT GHOSE, U.J. Idehenre, Yury Barnakov, S.A. Basun, D.R. Evans
Nanoscale BaTiO3 particles (10 nm) prepared by ball-milling a mixture of oleic acid and heptane have been reported to have an electric polarization several times larger than that for bulk BaTiO3. In this work, detailed local, intermediate, and long-range

Observations and identifications of extreme ultraviolet spectra of Ca-like to Na-like neodymium ions using an electron beam ion trap

August 23, 2023
Author(s)
Yang Yang, Dipti Dipti, Chihiro Suzukic, A. C. Gall, R. Silwal, Samuel Sanders, Joseph N. Tan, Aung S. Naing, Endre Takacs, Yuri Ralchenko
Extreme ultraviolet (EUV) radiation from M-shell Ca-like, Nd40+, through Nalike, Nd49+, highly charged ions have been measured at an electron beam ion trap (EBIT) facility at the National Institute of Standards and Technology. To produce the ionization

Mid-Infrared, Near-Infrared, and Visible Nanospectroscopy of Hydrogen-Intercalated MoO3

August 21, 2023
Author(s)
Jeffrey Schwartz, Sergiy Krylyuk, Devon Jakob, Albert Davydov, Andrea Centrone
Control over the local chemical composition and spatial heterogeneities in nanomaterials provides a means to impart new functions and to tailor their properties in many applications. For two-dimensional (2D) van der Waals materials, intercalation is one

MODELLING AND REMOVING DIGITIZER NONLINEARITY FOR ACCURATE DUAL FREQUENCY COMB SPECTROSCOPY

August 15, 2023
Author(s)
Nathan Malarich, Kevin Cossel, JEAN-DANIEL DESCHENES, Fabrizio Giorgetta, Brian Washburn, Nathan Newbury, Ian Coddington, Jerome Genest
Operation of any dual-comb spectrometer requires digitization of the interference signal before further processing. Nonlinearities in the analog-to-digital conversion can alter the apparent gas concentration by multiple percent, limiting both precision and

Imaging local luminescence variations in CdSe0.1Te0.9 thin films grown by the colossal grain growth process.

August 4, 2023
Author(s)
Ganga Neupane, Andrew Winchester, Nicolas Marquez Peraca, David Albin, Joel Duenow, Matthew Reese, Sujitra Pookpanratana, Susanna Thon, Behrang Hamadani
Clear visualization and understanding of luminescence properties of grain interiors and grain boundaries in polycrystalline thin-film photovoltaic materials are crucial to achieving high-performance solar cells. Luminescence-based measurements, for example

Synthetic Aperture RF Reception using Rydberg Atoms

August 2, 2023
Author(s)
Nik Prajapati, Aly Artusio-Glimpse, Matt Simons, Samuel Berweger, Drew Rotunno, Maitreyi Jayaseelan, Kaleb Campbell, Christopher L. Holloway
Rydberg atoms show great promise for use as self-calibrated electric field sensors for a broad range of frequencies. Their response is traceable to the international system of units making them a valuable tool for a variety of applications including

Titanium and titanium oxides at the K- and L-edges: comparing theoretical calculations to X-ray absorption and X-ray emission measurements

August 2, 2023
Author(s)
Karina Bzheumikhova, John Vinson, Ranier Unterumsberger, Malte Wansleben, Claudia Zech, Kai Schuler, Yves Kayser, Philipp Honicke, Burkhard Beckhoff
Using well-calibrated experimental data we demonstrate the applicability of theoretical X-ray absorption spectroscopy (XAS) as well as X-ray emission spectroscopy (XES) calculations for titanium (Ti), titanium oxide (TiO), and titanium dioxide (TiO2) at
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