June 1, 2017
      
                  
        
  Author(s)
  Nathan  Mahynski,   Lorenzo  Rovigatti,   Christos  Likos,   Athanassios  Panagiotopoulos
 
       
            
    
    
        We have used computer simulations to reveal how colloidal crystals may be assembled by engineering the shape and charge of polymeric additives, which act as structure-directing agents (SDAs). Using these agents, only a single desired polymorph may be