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Physics

Spectroscopy

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Displaying 476 - 500 of 1700

Real-time liquid-phase organic reaction monitoring with a mid-infrared dual frequency comb spectrometer

January 10, 2019
Author(s)
Daniel I. Herman, Eleanor M. Waxman, Gabriel G. Ycas, Fabrizio R. Giorgetta, Nathan R. Newbury, Ian R. Coddington
We combine high-resolution mid-infrared dual-comb spectroscopy with attenuated total reflectance measurements to provide in-situ monitoring of a chemical reaction. The mid-infrared dual-comb spectrometer measures quantitative absorption cross-sections of

Improving the Retrieval of XCO2 from Total Carbon Column Network Solar Spectra

January 3, 2019
Author(s)
Joseph Mendonca, Kimberly Strong, Debra Wunch, Geoffrey Toon, David Long, Joseph T. Hodges, Vincent T. Sironneau
High-resolution absorption spectra of the a^1 ∆_g←X^3 Σ_g^- O2 band measured using cavity ring-down spectroscopy were fitted using the Voigt and speed-dependent Voigt line shapes. We found that the speed-dependent Voigt line shape was better able to model

Measurement of Ion-Pairing Interactions in Buffer Solutions with Microwave Microfluidics

January 1, 2019
Author(s)
Charles A. Little, Angela C. Stelson, Nathan D. Orloff, Christian J. Long, James C. Booth
Broadband microwave microfluidics is an emerging technique for quantifying the frequency dependent electrical response of fluids in the microwave regime. This technique can access important physical properties including interfacial polarization, ion

Diagonal Slice Four-Wave Mixing: Natural Separation of Coherent Broadening Mechanisms

December 13, 2018
Author(s)
Travis M. Autry, Geoffrey M. Diederich, Mark E. Siemens
We present an ultrafast coherent spectroscopy data acquisition scheme that samples slices of the time domain used in multidimensional coherent spectroscopy to achieve faster data collection than full spectra. We derive analytical expressions for resonance

Multi-pulse fitting of transition edge sensor signals from a near-infrared continuous-wave source

December 11, 2018
Author(s)
Thomas Gerrits, Adriana E. Lita, Sae Woo Nam, Jianwei Lee, Lijiong Shen, Alessandro Cere, Christian Kurtsiefer
Transition-edge sensors (TESs) are photon-number resolving calorimetric spectrometers with near unit efficiency. Their recovery time, which is on the order of microseconds, limits the number resolving ability and timing accuracy in high photon-flux

Approximating vibronic spectroscopy with imperfect quantum optics

November 23, 2018
Author(s)
W.R. Clements, Jelmer Renema, Andreas Eckstein, Antonio A. Valido, Adriana Lita, Thomas Gerrits, Sae Woo Nam, Steven Kolthammer, Joonsuk Huh
We study the impact of experimental imperfections on a recently proposed protocol for performing quantum simulations of vibronic spectroscopy. Specifically, we propose a method for quantifying the impact of these imperfections, optimizing an experiment to

Gain Calibration of Current-to-Voltage Converters

November 19, 2018
Author(s)
Thomas C. Larason, Carl C. Miller
Current-to-voltage converters are used in many photometric and radiometric applications. The calibration of current- to-voltage converters at a few input currents is not always sufficient to understand the linearity and the bias of a device. Many devices

Dephasing of InAs quantum dot p-shell excitons using two-dimensional coherent spectroscopy

November 12, 2018
Author(s)
Galan Moody, Takeshi Suzuki, Rohan Singh, Marc Assman, Manfred Bayer, Arne Ludwig, Andreas Wieck, Steven T. Cundiff
The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects

In aqua electrochemistry probed by XPEEM: experimental setup, examples, and challenges

November 10, 2018
Author(s)
Slavomir Nemsak, Evgheni Strelcov, Hongxuan Guo, Brian Hoskins, Tomas Duchon, D Muller, Alexander Yulaev, Ivan Vlassiouk, Alexander Tselev, Andrei Kolmakov
Recent developments in environmental and liquid cells equipped with electron transparent graphene windows have enabled traditional surface science spectromicroscopy tools, such as XPS, PEEM, and SEM to be applied to study solid-liquid and liquid-gas
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