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Studies and calibrations of short-lived radionuclides, for example 15O, are of particular interest in nuclear medicine. Yet counting experiments on such species are vulnerable to an error due to the combined effect of decay and dead time. Separate decay
The β-γ anticoincidence method is used for the primary standardization of β-, β+, electron capture (EC), α, and mixed-mode radionuclides. Efficiency extrapolation using one or more γ ray coincidence gates is typically carried out by a low-order polynomial
One material attribute for nuclear forensics is material age. 241Pu is almost always present in uranium- and plutonium-based nuclear weapons, which pose the greatest threat to our security. The in-growth of 241Am due to the decay of 241Pu provides an
Ronald Colle, Ryan P. Fitzgerald, Lizbeth Laureano-Perez
Ultra-pure, carrier-free 209Po solution standards have been prepared and standardized for their massic alpha-particle emission rate. The standards, which will be disseminated by the National Institute of Standards and Technology (NIST) as Standard
Collé, et al [(2007) Appl. Radiat Isot. 65, 728; (2014) J. Phys. G: Nucl. Part. Phys. 41, 105103], over the course of nearly a decade and with decay data from a period of 20.7 years, initially uncovered and then substantiated a 25 % error in the 209Po half
Ryan P. Fitzgerald, Claude Bailat, Christophe Bobin, John Keightley
The 4-pi-beta-gamma coincidence counting method and its close relatives are widely used for the primary standardization of radioactivity. Both the general formalism and specific implementation of these methods have been well-documented. In particular, the
Marie Noelle Amiot, V Chiste, Ryan P. Fitzgerald, F Juget, Carine Michotte, Andrew Pearce, G Ratel
Pressurized re-entrant (or 4π) pressurized ionization chambers (ICs) connected to current- measuring electronics are used for activity measurements of photon emitting radionuclides and some beta emitters in the field of metrology and nuclear medicine. As a
Nuclear counting is affected by pulse pileup and system dead time which induce rate-related count loss and alter the statistical properties of the counting process. Fundamental equations are presented to predict deviations from Poisson statistics due to
Ra-223 is an alpha-emitter that is being used as a bone-seeking radiotherapeutic agent. The relatively large uncertainty on its half-life (0.26 %, Bé et al., 2011) is an impediment to precision activity assays. We have performed two series of measurements
Denis E. Bergeron, Jeffrey T. Cessna, Brian E. Zimmerman
Dose calibrator dial settings reported by NIST in 2010 (ARI v. 68, p. 1367) are now known to give erroneously low (by 10 %) activity readings. The original determinations were based on a chain of calibrations; a broken link in this chain was recently
The cryogenic design and performance of an apparatus used to magnetically confine ultracold neutrons (UCN) is presented. The apparatus is part of an effort to measure the beta-decay lifetime of the free neutron and is comprised of a high-current supercon-
The critical micelle concentration and the phase boundary between isolated surfactant molecules and aggregates are probed via fluorescence spectroscopy and a Compton spectrum quenching technique for aqueous and toluenic solutions of Triton X-100 (TX-100)
Denis E. Bergeron, Jeffrey T. Cessna, Bert M. Coursey, Ryan P. Fitzgerald, Brian E. Zimmerman
The new NIST activity standardization for 18F differs from results obtained between 1998 and 2008 by 4 %. The new results are considered to be very reliable; they are based on a battery of robust primary measurement techniques and bring the NIST standard
Ronald Colle, Ryan P. Fitzgerald, Lizbeth Laureano-Perez
A substantial 25 % error in the then known and accepted (102 5) year half-life of 209Po was reported on in 2007. This error was detected from decay data from two separate primary standardizations of a 209Po solution standard, which were performed
Hans P. Mumm, Alan Keith Thompson, Paul R. Huffman, Christopher O'Shaughnessy, Kevin J. Coakley, Robert Golub, John M. Doyle, Steve K. Lamoreaux, P.-N. Seo, C E. Mattoni, S N. Dzhosyuk, L Yang, Grace L. Yang, Karl W. Schelhammer, Christopher M. Swank
The neutron beta-decay lifetime plays an important role, both in understanding weak interactions within the framework of the Standard Model, and in theoretical predictions of the primordial abundance of 4He in Big Bang Nucleosynthesis. In previous work, we
We describe an experiment to measure the neutron lifetime using a technique with a set of systematic uncertainties largely different than those of previous measurements. In this approach, UCN are produced by inelastic scattering of cold (0.89 nm) neutrons
Reactor antineutrino experiments have the ability to search for neutrino oscillations independent of reactor flux predictions using a relative measurement of the neutrino flux and spectrum across a range of baselines. The range of accessible oscillation
Reactor antineutrinos are used to study neutrino oscillation, search for signatures of non-standard neutrino interactions, and to monitor reactor operation for safeguard applications. The flux and energy spectrum of reactor antineutrinos can be predicted
W. Zheng et al. [Phys. Rev. A 83, 061401(R) (2011)] measure under certain conditions a linear pressure dependence of the wall-induced nuclear relaxation rate of 3He in glass cells typically used to generate and/or store hyperpolarized 3He. Their
Brian E. Zimmerman, Denis E. Bergeron, Jeffrey T. Cessna
An international Key Comparison of 177Lu has recently been carried out. Twelve laboratories performed assays for radioactivity content on aliquots of a common master solution of 177Lu, leading to eleven results submitted for entry into the Key Comparison
For over 30 years scientists in the NIST radioactivity group have been using their ionization chamber A to make measurements of radioactivity and radioactive half-lives. We now have evidence that some of those reported measurements were incorrect due to
Various theories beyond the Standard Model predict new particles with masses in the sub-eV range with very weak couplings to ordinary matter. A P-odd, T-odd, spin-dependent interaction between polarized and unpolarized matter is one such possibility. Such
The wall effect in liquid scintillation (LS) counting is the loss of efficiency in the case that an alpha-particle hits a surface (wall or air) before depositing enough energy to be detected. We report our measurements of this LS inefficiency using the 4
A M. Micherdzinska, C. D. Bass, T. D. Bass, K. F. Gan, D Lou, D M. Markoff, Hans Pieter Mumm, Jeffrey S. Nico, A. K. Opper, E I. Sharapov, M Snow, H E. Swanson, V Zhumabekova
Measurements of parity-violating neutron spin rotation can provide insight into the poorly nderstood nucleon-nucleon weak interaction. Because the expected rotation angle per unit length is small (10−7 rad/m), several properties of the polarized cold
Nuclear magnetic resonance gyroscopes(NMRGs)detect rotation as shift in the Larmor precession frequency of nuclear spins. A review of the open literature on NMRGs is presented, which includes an introduction to the spectroscopic techniques that enable