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Displaying 51 - 75 of 141

Sub-picosecond charge-transfer at near-zero driving force in polymer:non-fullerene acceptor blends and bilayers

February 11, 2020
Author(s)
Yufei Zhong, Martina Causa, Gareth J. Moore, Philipp Krauspe, Bo Xiao, Jonas Kublitski, Rishi Shivhare, Johannes Benduhn, Eyal BarOr, Subhrangsu Mukherjee, Kaila Yallum, Julien R?hault, Stefan C. Mannsfeld, Dieter Neher, Lee J. Richter, Dean DeLongchamp, Frank Ortmann, Koen Vandewal, Erjun Zhou, Banerji Natalie, Florian Gunther
Organic photovoltaics based on non-fullerene acceptors (NFAs) show record efficiency of 16 to 17% and increased photovoltage owing to the low driving force for interfacial charge-transfer. However, the low driving force potentially slows down charge

Influence of Polymer Aggregation and Liquid Immiscibility on Morphology Tuning by Varying Composition in PffBT4T-2DT/Non-Fullerene Organic Solar Cells

January 29, 2020
Author(s)
Subhrangsu Mukherjee, Dean M. DeLongchamp, Regis J. Kline, Iain McCulloch, Zeinab Hamid, Andrew Wadsworth, Elham Rezasoltani, Sarah Holliday, Mohammed Azzouzi, Anne Guilbert, Yifan Dong, Marios Neophytou, Mark Little, Helen Bristow, Artem Bakulin, James Durrant, Jenny Nelson, Andrew A. Herzing
The temperature dependent aggregation behavior of PffBT4T polymers used in organic solar cells plays a critical role in the formation of a favorable morphology in fullerene-based devices. However, there has been little investigation into the impact of

Nonvolatile memory based on redox-active Ruthenium molecular monolayers

October 14, 2019
Author(s)
Kai Jiang, Sujitra Pookpanratana, Tong Ren, Sean Natoli, Brent A. Sperling, Joseph W. Robertson, Curt A. Richter, Sheng Yu, Qiliang Li
A monolayer of diruthenium molecules was self-assembled onto the silicon oxide surface in a semiconductor capacitor structure with a ‘click' reaction for nonvolatile memory applications. The attachment of the active molecular monolayer was verified by x

Photovoltaic Blend Microstructure for High Efficiency Post-Fullerene Solar Cells. To Tilt or Not To Tilt?

August 5, 2019
Author(s)
Subhrangsu Mukherjee, Dean M. DeLongchamp, Gang Wang, Steven M. Swick, Micaela Matta, Joseph Strzalka, Thomas Aldrich, Ferdinand Melkonyan, Antonio Facchetti, Tobin Marks, Jenna L. Logsdon, Simone Fabiano, Wei Huang, Tony Yang, Amod Timalsina, Natalia Powers-Riggs, Joaquin Alzola, Ryan M. Young, Michael R. Wasielewski, George C. Schatz
Achieving efficient polymer solar cells (PSCs) requires a structurally optimal donor–acceptor heterojunction morphology. Here we report the combined experimental and theoretical characterization of a benzodithiophene–benzothiadiazole donor polymer series

Correlating anisotropic mobility and intermolecular phonons in organic semiconductors to investigate transient localization

March 19, 2019
Author(s)
Emily G. Bittle, Adam J. Biacchi, Lisa A. Fredin, Andrew A. Herzing, Thomas C. Allison, Angela R. Hight Walker, David J. Gundlach
Charge transport in organic semiconductors is governed by a mix of polaron hopping and band- like transport mechanisms. The energy of polaron hopping and formation are similar in magnitude to the energies of inter- and intra- molecular modes, which points

Higher Order Effects in Organic LEDs with Sub-bandgap Turn-on

January 16, 2019
Author(s)
Sebastian Engmann, Adam J. Barito, Emily Bittle, Chris Giebink, Lee J. Richter, David J. Gundlach
Spin-dependent nonlinear processes in organic materials such as singlet-fission and triplet- triplet annihilation could increase the performance for photovoltaics, detectors, and light emitting diodes. Rubrene/C60 light emitting diodes exhibit a distinct

Electrical Detection of Singlet Fission in Single Crystal Tetracene Transistors

January 4, 2019
Author(s)
Hyuk-Jae Jang, Emily Bittle, Qin Zhang, Adam Biacchi, Curt A. Richter, David J. Gundlach
Here, we present the electrical detection of singlet fission in tetracene by using a field- effect transistor (FET). Singlet fission is a photo-induced spin-dependent process yielding two triplet excitons from the absorption of a single photon. , In this

A simple and robust approach to reducing contact resistance in organic devices

December 3, 2018
Author(s)
Lamport Zachary, Katrina Barth, Hyunsu Lee, Martin Guthold, Iain McCulloch, John E. Anthony, Lee J. Richter, Eliot Gann, Dean DeLongchamp, Oana Jurchescu
Efficient injection of charge carriers from the contacts into the semiconductor layer is crucial for achieving high-performance organic devices. The potential drop necessary to accomplish this process yields a resistance associated with the contacts
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