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Physics

Spectroscopy

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  • Published Date
Displaying 301 - 325 of 911

Approximating vibronic spectroscopy with imperfect quantum optics

November 23, 2018
Author(s)
W.R. Clements, Jelmer Renema, Andreas Eckstein, Antonio A. Valido, Adriana Lita, Thomas Gerrits, Sae Woo Nam, Steven Kolthammer, Joonsuk Huh
We study the impact of experimental imperfections on a recently proposed protocol for performing quantum simulations of vibronic spectroscopy. Specifically, we propose a method for quantifying the impact of these imperfections, optimizing an experiment to

Gain Calibration of Current-to-Voltage Converters

November 19, 2018
Author(s)
Thomas C. Larason, Carl C. Miller
Current-to-voltage converters are used in many photometric and radiometric applications. The calibration of current- to-voltage converters at a few input currents is not always sufficient to understand the linearity and the bias of a device. Many devices

Dephasing of InAs quantum dot p-shell excitons using two-dimensional coherent spectroscopy

November 12, 2018
Author(s)
Galan Moody, Takeshi Suzuki, Rohan Singh, Marc Assman, Manfred Bayer, Arne Ludwig, Andreas Wieck, Steven T. Cundiff
The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects

In aqua electrochemistry probed by XPEEM: experimental setup, examples, and challenges

November 10, 2018
Author(s)
Slavomir Nemsak, Evgheni Strelcov, Hongxuan Guo, Brian Hoskins, Tomas Duchon, D Muller, Alexander Yulaev, Ivan Vlassiouk, Alexander Tselev, Andrei Kolmakov
Recent developments in environmental and liquid cells equipped with electron transparent graphene windows have enabled traditional surface science spectromicroscopy tools, such as XPS, PEEM, and SEM to be applied to study solid-liquid and liquid-gas

Contact and Non-Contact Measurement of Electronic Transport in Individual 2D SnS Colloidal Semiconductor Nanocrystals

September 24, 2018
Author(s)
Adam J. Biacchi, Son T. Le, Brian G. Alberding, Joseph A. Hagmann, Sujitra J. Pookpanratana, Edwin J. Heilweil, Curt A. Richter, Angela R. Hight Walker
Colloidal-based solution syntheses offer a scalable and cost-efficient means of producing 2D nanomaterials in high yield. While much progress has been made towards the controlled and tailorable synthesis of semiconductor nanocrystals in solution, it

Flow-induced crystallization during materials extrusion additive manufacturing

September 10, 2018
Author(s)
Lily Northcutt, Sara Orski, Kalman D. Migler, Anthony Kotula
Material extrusion additive manufacturing processes force molten polymer through a printer nozzle at high (> 100 s-1) wall shear rates prior to cooling and crystallization. These high shear rates can lead to flow-induced crystallization in common polymer

Optical Properties of Meloxicam in the Far-Infrared Spectral Region

August 17, 2018
Author(s)
Yusuf S. Aytekin, Mustafa Koturk, Adam Zaczek, Timothy M. Korter, Edwin J. Heilweil, Okan Esenturk
One of the most commonly used nonsteroidal anti-inflammatory active pharmaceutical ingredient called Meloxicam has been characterized spectroscopically both by Terahertz (THz) time domain spectroscopy (THz-TDS) and by Fourier Transform Infrared (FTIR)

Photochemical Dynamics of a Trimethyl-Phosphine Derivatized [FeFe]-Hydrogenase Model Compound

August 17, 2018
Author(s)
Edwin J. Heilweil, Rachel L. Meyer, Tara M. Biser, Anet D. Zhandosova, Christopher J. Stromberg
Coupling photosensitizers with [FeFe]-hydrogenase model compounds can potentially create light- driven catalysts for production of hydrogen gas from acidic protons. Though there have been many studies on the synthesis, kinetics, and reaction mechanisms of

Chemical Compound Classification by Elemental Signatures in Castle Dust Using SEM Automated X-ray Particle Analysis

August 1, 2018
Author(s)
Diana Ortiz-Montalvo, Edward P. Vicenzi, Nicholas W. Ritchie, Carol A. Grissom, Richard A. Livingston, Zoe Weldon-Yochim, Joseph M. Conny, Scott A. Wight
Discoloration on the Smithsonian Institution Building and Enid A. Haupt Garden gateposts was recently revealed to be related to a Mn enriched rock varnish. Mn does not appear to be derived locally from the building stone; therefore, its source is likely

Characterization of Interfacial Structure in Polymer-Fullerene Bulk Heterojunctions via 13C {2H} Rotational Echo Double Resonance NMR

July 13, 2018
Author(s)
Ryan C. Nieuwendaal, Dean M. DeLongchamp, Martin Heeney, Jan Hummelen, Chad R. Snyder, Ronald L. Jones, Sebastian Engmann, Lee J. Richter, Zhuping Fei, Alex Sieval
We introduce a new application of solid state NMR measurements towards characterizing the donor-acceptor interfaces within bulk heterojunction (BHJ) films. Rotational echo double resonance (REDOR) is used to measure dipolar couplings between 13C nuclei on

A Scalable Readout for Microwave SQUID Multiplexing of Transition-Edge Sensors

July 9, 2018
Author(s)
Johnathon D. Gard, Daniel T. Becker, Douglas A. Bennett, Joseph W. Fowler, Gene C. Hilton, John A. Mates, Carl D. Reintsema, Daniel R. Schmidt, Daniel S. Swetz, Joel N. Ullom
The readout requirements for instruments based on transition-edge sensors (TESs) have dramatically increased over the last decade as demand for systems with larger arrays and faster sensors has grown. Emerging systems are expected to contain many thousands

Electronic Properties and Structure of Single Crystal Perylene

June 6, 2018
Author(s)
Sujitra J. Pookpanratana, Katelyn Goetz, Emily G. Bittle, Hamna Haneef, Lin You, Christina A. Hacker, Steven W. Robey, Oana Jurchescu, Ruslan Ovsyannikov, Erika Giangrisostomi
The transport properties of electronic devices made from single crystalline molecular semiconductors outperform those composed of thin-films. To further understand the superiority of these extrinsic properties, an understanding of the intrinsic electronic

Imaging linear and circular polarization features in leaves with complete Mueller matrix polarimetry

June 1, 2018
Author(s)
C.H. L. Patty, David Luo, Frans Snik, Freek Ariese, Wybren J. Buma, Inge L. ten Kate, Rob J. van Spanning, William Sparks, Thomas Germer, Gy?z? Garab, Michael W. Kudenov
Spectropolarimetry of intact plant leaves allows to probe the molecular architecture of vegetation photosynthesis in a non-invasive and non-destructive way and, as such, can offer a wealth of physiological information. In addition to the molecular signals

Nanoscale photocurrent mapping in perovskite solar cells

June 1, 2018
Author(s)
Yohan Yoon, Dongheon Ha, Ik Jae Park, Paul M. Haney, Sangwook Lee, Nikolai Zhitenev
In this work, we study spatially-resolved generation of photocurrent of methylammonium lead iodide (CH3NH3PbI3) perovskite solar cells to reveal the microscopic effects of annealing temperature and degradation under light exposure. Correlating a novel
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