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Primary Standardization of Radionuclides by Anticoincidence Counting

Summary

The standardization of radionuclides by primary methods is the foundation for all the standards and services provided by the NIST radioactivity group.

Description

Monte-Carlo simulation
Credit: Ryan P. Fitzgerald

Monte-Carlo simulation of NIST live-timed anticoincidence system. Simulation and experiment are combined to achieve high accuracy in the primary standardization of electron capture radionuclides.

These include: SRM's, calibrations, and proficiency testing. A principle method of primary standardization at NIST is live-timed 4πβ-γ anticoincidence counting (LTAC). Using this technique, researchers at NIST have recently developed standards for nuclear imaging (18F), cancer treatment (223Ra), and nuclear forensics (241Pu/241Am chronometer).

Primary standards for various radionuclides based on LTAC have been submitted to international comparisons and have been found to be in excellent agreement with other national metrology institutes. Furthermore, NIST researchers use these primary standards to calibrate their own secondary instruments, including ionization chambers and γ-ray spectrometers.

Recent work, presented at the International Conference on Radionuclide Metrology and its Applications (ICRM), includes improvement in accuracy by incorporating GEANT4-based Monte Carlo simulations into efficiency extrapolations, as well as the development of a digital electronics chain for list-mode analysis.

Created April 14, 2011, Updated January 23, 2018