An official website of the United States government
Here’s how you know
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
Secure .gov websites use HTTPS
A lock (
) or https:// means you’ve safely connected to the .gov website. Share sensitive information only on official, secure websites.
We consider a two-state system driven by an on-resonance, continuous wave pump laser and a much weaker pulsed probe laser that is slightly detuned from the pump laser frequency usually this detuning is about p −P=1 kHz. The upper state population is
We investigate an active Raman gain scheme for significant group velocity reduction. We show that this scheme, which is fundamentally different from the electromagnetically induced transparency scheme, is capable of achieving ultraslow and distortion-free
We study the formation of a nonlinear localized high-dimensional optical beam in a lifetime- broadened three-state atomic system. We show that stable high-dimensional spatial optical solitons with extremely weaklight intensity can occur in such a highly
Neil A. Anderson, Lee J. Richter, John C. Stephenson, Kimberly A. Briggman
The main gel to liquid crystal (LC) phase transition temperature, Tm, of the lipid monolayers in hybrid bilayer membranes (HBMs) was investigated using vibrational sum frequency spectroscopy (VSFS). The unique sensitivity of VSFS to probe order/disorder
We present a portable spectrometer that uses the frequency-stabilized cavity ring-down spectroscopy technique to realize high-precision measurements of trace water vapor concentration. Measuring one of the strongest rovibrational transitions in the 1 + 3
Broadband coherent anti-Stokes Raman spectroscopy (CARS) is demonstrated as an effective probe of the polymer thin film materials. A simple modification to a commercially available 1 kHz SFG spectrometer permits acquisition of CARS spectra for polymer thin
Christopher D. Zangmeister, Steven W. Robey, Roger D. van Zee
Photoelectron spectroscopy was used to explore changes in Fermi level alignment, within the p-p* gap, arising from changes in the coupling chemistry of conjugated phenylene ethynlene oligomers to the Au surface. Self-assembled monolayers were formed
We study stable propagation of multiple shape-preserving optical pulses in an inhomogeneously broadened multi-level atomic medium. By analytically solving the Maxwell-Schr¿odinger equations governing the evolution of N coupled optical fields and atomic
A measurement of the natural linewidth of the 401 nm 4f 126s 2 ( 3H 6) {rarr} 4f 12( 3H)6s6p ( 1P o 1) (6,1) 7 o transition in Er I is presented. Using laser-induced fluorescence in an atomic beam, a linewidth of (36.0 {plus or minus} 1.2) MHz is observed
Lu Deng, M. G. Payne, Guoxiang Huang, kaijun Jiang
We investigate the simultaneous formation and propagation of coupled ultraslow optical soliton pairs in a cold, lifetime-broadened three-state double- atomic system. Starting from the equations of motion of atomic response and two-mode probe-control
In studies of various nonlinear optical phenomena, strong resonant features in the atomic or molecular response to multi-photon driven processes have been used to greatly enhance the visibility of otherwise weak higher- order processes. However, there are
K D. Ridge, N G. Abdulaev, Xi-Cheng Zhang, T Ngo, D M. Brabazon, John P. Marino
Solution NMR studies of a 15N-labeled G-protein ?-subunit (G?) chimera (15N-ChiT) reconstituted heterotrimer have previously shown that binding of ??-subunits induces a pre-activated conformation in G? that may facilitate interaction with R* and guanine
We investigate the influence of high-order dispersion and nonlinearity on the propagation of ultraslow optical solitons in a lifetime broadened four-state atomic system under a Raman excitation. Using a standard method of multiple-scales we derive a
We investigate a life time broadened and coherently prepared five-state system for multi-wave mixing processes. We show that very efficient wave mixing occurs, producing an unconventional mixing wave that has the characteristics of both conventional four
We present a portable spectrometer that uses the frequency-stabilized cavity ring-down spectroscopy technique to realize high-precision measurements of trace water vapor concentration. Measuring one of the strongest rovibrational transitions in the 1 + 3
Laura B. Picraux, Christopher D. Zangmeister, J Batteas
This study investigates the formation of low-density, flat-lying decanethiol chemisorbed on Au prepared by heating the surface covered with a densely-packed, upright monolayer to a surface temperature above the onset of desorption. We determined conditions
David L. Duewer, John C. Travis, J. C. Acosta, G Andor, J Bastie, P. Blattner, C J. Chunnilall, S. C. Crosson, E. A. Early, F. Hengstberger, C. Kim, L. Liedquist, F Manoocheri, A. Mito, L.A. G. Monard, S Nevas, M. Nilsson, M Noel, A C. Rodriguez, A Ruiz, A. Schirmacher, M V. Smith, G. Valencia, N. van Tonder, Joanne C. Zwinkels
H Ban, M Jacka, James L. Hanssen, Joseph Reader, Jabez J. McClelland
We discuss laser cooling opportunities in atomic erbium, identifying five J rarr} J + 1 transitions from the 4f 126s 2 3H 6 ground state that are accessible to common visible and near-infrared continuous-wave tunable lasers. We present lifetime
M Bartenstein, A Altmeyer, S Riedl, R Geursen, S Jochim, C Chin, J Hecker Denschlag, R Grimm, Andrea Simoni, Eite Tiesinga, Carl J. Williams, Paul S. Julienne
Radio-frequency spectroscopy on weakly bound 6Li_2 molecules determines to high precision the molecular binding energies and the energy splitting between molecular states. By fitting the measurement to a multi-channel quantum scattering model, we determine
We show that in a two-mode, three-level, double-L system an efficient multiphoton destructive interference involving one- and three-photon pumping pathways occurs, leading to a unique type of induced transparency. Unlike the conventional
Both infrared and Raman are increasingly applied in biomolecular structure characterization, thus getting acceptance alongside traditional bioanalytical techniques. Physical principles and biological sampling requirements are reviewed. Advanced
We analyze a lifetime-broadened four-state four-wave-mixing (FWM) scheme in the ultraslow propagation regime and show that the generated FWM field can acquire the same group velocity and pulse shape as those of an ultraslow pump field. We show that a new