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Physics

Spectroscopy

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Displaying 676 - 700 of 927

Amplification of the optical absorption cross section for aerosols of soot with a nonabsorbing coating from photoacoustic measurements

May 13, 2011
Author(s)
Pedro Bueno, Daniel K. Havey, George W. Mulholland, Joseph T. Hodges, Keith A. Gillis, Russell R. Dickerson, Michael R. Zachariah
A quantitative understanding of the absorption and scattering properties of mixed soot and aerosol particles is necessary for evaluating the Earth's energy balance. Uncertainty in the net radiative forcing of atmospheric aerosols is relatively large and

Recent developments in the NIST Atomic Databases

May 11, 2011
Author(s)
Alexander Kramida
New versions of the NIST Atomic Spectra Database (ASD, v. 4.0) and three bibliographic databases (Atomic Energy Levels and Spectra, v. 2.0, Atomic Transition Probabilities, v. 9.0, and Atomic Line Broadening and Shapes, v. 3.0) have recently been released

Characterization of the First Order Nonlinear Stiffened Elasticity of the Piezoelectric Layer in Bulk Acoustic Wave Resonators

May 1, 2011
Author(s)
Juan C. Collado Gomez, Eduard Rocas, Jordi Mateu, Nathan D. Orloff, James C. Booth, Alberto Padillo, Juan Callaghan
This work proposes a procedure to characterize the intrinsic nonlinearities of bulk acoustic wave resonators by performing one port measurements of the second harmonic and second order intermodulation spurious signals. Closed-form expressions have been

Dual comb spectroscopy from 1.25 to 1.7 ym

May 1, 2011
Author(s)
Alexander M. Zolot, Ian R. Coddington, Fabrizio R. Giorgetta, Esther Baumann, William C. Swann, Nathan R. Newbury
A coherent dual comb spectrometer spanning much of the near infrared was constructed from broadened erbium fiber lasers. Gas phase water, methane and acetylene spectra were measured and characterized toward establishing new frequency standards.

Conformer-specific vibronic spectroscopy and vibronic coupling in a flexible bichromophore: bis-(4-hydroxyphenyl)methane

April 28, 2011
Author(s)
Chirantha P. Rodrigo, Christian Muller, Nathan Pillsbury, William H. James III, David F. Plusquellic, Timothy Zwier
The vibronic spectroscopy of jet-cooled bis-(4-hydroxyphenyl)methane (b4HPM) has been explored using fluorescence excitation (FE), dispersed fluorescence (DFL), UV-UV holeburning (UVHB), UV depletion (UVD), and fluorescence-dip infrared (FDIR)

Chirped-pulse terahertz spectroscopy for broadband trace gas sensing

April 22, 2011
Author(s)
Eyal Gerecht, Kevin O. Douglass, David F. Plusquellic
We report the first demonstration of a broadband trace gas sensor based on chirp-pulse terahertz spectroscopy. The advent of newly developed solid state sources and heterodyne detectors for the terahertz frequency range have made it possible to generate

Searching for applications with a fine-toothed comb

April 1, 2011
Author(s)
Nathan R. Newbury
Frequency combs, like many ground-breaking technologies, are simple in concept; they results from the spectrum of any regular train of optical pulses. What is remarkable is that this simple picture can be actually realized in a number of different

X-ray Emission Spectroscopy of Nitrogen-rich Compounds

March 31, 2011
Author(s)
Terrence J. Jach, Fernando D. Vila, W. T. Elam, J. D. Denlinger, John J. Rehr
Non-resonant x-ray emission spectroscopy was used to compare the nitrogen-rich compounds ammonium nitrate, trinitrotoluene, and cyclotrimethylene-trinitramine. They are representative of crystalline and molecular structures of special importance in

Quantification and Compensation of Unintentional Analyte Aggregation in Electrospray Sampling

March 30, 2011
Author(s)
Mingdong M. Li, Suvajyoti S. Guha, Rebecca A. Zangmeister, Michael J. Tarlov, Michael R. Zachariah
Electrospray (ES) sources are commonly used to introduce non-volatile materials (e.g. nanoparticles, proteins, etc.) in to the gas phase for characterization by mass spectrometry and ion mobility. Recent studies in our group using electrospray ion mobility

High Accuracy Measurements of OH Reaction Rate Constants and IR and UV Absorption Spectra: Ethanol and Partially Fluorinated Ethyl Alcohols.

March 4, 2011
Author(s)
Vladimir L. Orkin, Victor Khamaganov, Larissa E. Martynova, Michael J. Kurylo III
Rate constants for the gas phase reactions of OH radicals with ethanol and three fluorinated ethyl alcohols, CH3CH2OH (k0), CH2FCH2OH (k1), CHF2CH2OH (k2), and CF3CH2OH (k3) were measured using a flash photolysis resonance-fluorescence technique over the

Differential Light Shift Cancellation in a B-Field Insensitive Transition of 87Rb

February 11, 2011
Author(s)
Radu S. Chicireanu, Karl D. Nelson, Steven M. Olmschenk, Nathan Lundblad, A. Derevianko, James V. Porto
We demonstrate substantial cancellation of the differential light shift of a magnetic-field-insensitive microwave hyperfine (clock) transition in 87Rb atoms trapped in an optical lattice. Up to 95.5% of the differential light shift is cancelled while

Comparison of the Sensitivity and Image Contrast in Spontaneous Raman and Coherent Stokes Raman Scattering Microscopy of Geometry Controlled Samples

February 9, 2011
Author(s)
Hyun M. Kim, Chris A. Michaels, Garnett W. Bryant, Stephan J. Stranick
We experimentally compare the performance and contrast differences between spontaneous and coherent Stokes Raman scattering microscopy. We demonstrate the differences on a series of geometry controlled samples that range in complexity from a point (array

Passive Intermodulation due to Self-Heating in Printed Transmission Lines*

February 2, 2011
Author(s)
Eduard Rocas, Juan C. Collado Gomez, Nathan D. Orloff, Jordi Mateu, James C. Booth, Juan M. O'Callaghan, Alberto Padilla
Abstract—This article proposes a mechanism by which third-order intermodulation distortion due to self-heating is generated in transmission lines. The work shows how transmission lines made of several materials whose properties are independent of the

Approximate theoretical model for the five electronic states (? = 5/2, 3/2, 3/2, 1/2, 1/2) arising from the ground 3d9 configuration in nickel halide molecules and for the rotational levels of the two ? = 1/2 states in this manifold

January 25, 2011
Author(s)
Jon T. Hougen
This paper is divided into two parts. In the first part an effective Hamiltonian for a non-rotating diatomic molecule containing only crystal-field and spin-orbit operators is set up to describe the energies of the five spin-orbit components that arise in

Performance of a coherent dual frequency comb spectrometer

January 1, 2011
Author(s)
Nathan R. Newbury, Esther Baumann, Ian R. Coddington, Fabrizio R. Giorgetta, William C. Swann, Alexander M. Zolot
We discuss the performance of a coherent dual frequency comb spectrometer in terms of signal-to-noise ratio, resolution, and accuracy based on experimental data in the near and short-wave infrared centered at 1.5 and 3.4 micrometers.

Progress at NIST in measuring the D-lines of Li isotopes using an optical frequency comb

December 20, 2010
Author(s)
Clayton Simien, Samuel M. Brewer, Joseph N. Tan, John D. Gillaspy, Craig J. Sansonetti
Precise spectroscopic experiments with light atoms can provide information about nuclear properties that are very difficult to obtain in electron scattering experiments. For example, relative nuclear radii of low-Z isotopes can be determined accurately
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