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Physics

Condensed matter

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Displaying 276 - 300 of 1253

Evaluating the Effects of Structural Disorder on the Magnetic Properties of Nd 2 Zr 2 O 7

August 9, 2021
Author(s)
Eli Zoghlin, Julian Schmehr, Collin Holgate, Rebecca Dally, Yaohua Liu, Geneva Laurita, Stephen Wilson
Motivated by the variation in reported lattice parameters of floating-zone-grown Nd 2Zr 2O 7 crystals, we have performed a detailed study of the relationship between synthesis environment, structural disorder, and magnetic properties. Using a combination

Evolution of Magnetic Interactions in Sb-Substituted MnBi 2 Te 4

August 2, 2021
Author(s)
S. Riberolles, Q. Zhang, Elijah Gordon, Nicholas Butch, Liqin Ke, J.-Q. Yan, R. McQueeney
The Mn(Bi 1−xSb x) 2Te 4 series is purported to span from antiferromagnetic (AF) topological insulator at x = 0 to a trivial AF insulator at x = 1. Here we report on neutron diffraction and inelastic neutron scattering studies of the magnetic interactions

De-excitation dynamics of muonic atoms revealed by high precision spectroscopy of electronic K x rays using a superconducting transition-edge sensor microcalorimeter

July 27, 2021
Author(s)
Douglas Bennett, W.Bertrand (Randy) Doriese, Malcolm Durkin, Joseph Fowler, Johnathon Gard, Gene C. Hilton, Kelsey Morgan, Galen O'Neil, Carl D. Reintsema, Dan Schmidt, Daniel Swetz, Joel Ullom, Toshiyuki Azuma, Pietro Caradonna, I-Huan Chiu, Tadashi Hashimoto, Ryota Hayakawa, Yuto Ichinohe, Paul Indelicato, TadaAki Isobe, Sohtaro Kanda, Daiji Kato, Miho Katsuragawa, Naritoshi Kawamura, Yasushi Kino, Kenya Kubo, Kairi Mine, Yasuhiro Miyake, Kazuhiko Ninomiya, Hirofumi Noda, Shinji Okada, Takuma Okumura, Kenichi Okutsu, Takahito Osawa, Nancy Paul, Kouichiro Shimomura, Patrick Strasser, Hirotaka Suda, Tadayuki Takahashi, Shinichiro Takeda, Soshi Takeshita, Motonobu Tampo, Hideyuki Tatsuno, XiaoMin Tong, Yasuhiro Ueno, Shin Watanabe, Shinya Yamada
We observed electronic K x rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic

Magnetic Structure, Excitations and Short-Range order in Honeycomb Na 2 Ni 2 TeO 6

July 15, 2021
Author(s)
Nathan Episcopo, Po-Hao Chang, Thomas W. Heitmann, Kinley Wangmo, James M. Guthrie, Magdalena Fitta, Ryan Klein, Narayan Poudel, Krzysztof Gofryk, Rajendra R. Zope, Craig Brown, Harikrishnan S. Nair
Na 2Ni 2TeO 6 has a layered hexagonal structure with a honeycomb lattice constituted by Ni 2+ and a chiral charge distribution of Na + that resides between the Ni layers. In the present work, the antiferromagnetic transition temperature of Na 2Ni 2TeO 6 is

Dynamic Crossover in Fluids: From Hard Spheres to Molecules

July 7, 2021
Author(s)
Ian Bell, Stephanie Delage-Santacreu, Hai Hoang, Guillaume Galliero
We propose a simple and generic definition of a demarcation reconciling structural and dynamic frameworks when combined with the entropy scaling framework. This crossover line between gas- and liquid-like behaviors is defined as the curve for which an

Coulombically-stabilized oxygen hole polarons enable fully reversible oxygen redox

July 1, 2021
Author(s)
Iwnetim I. Abate, Chaitanya D. Pemmaraju, Se-Young Kim, Sami Sainio, Brian Moritz, John Vinson, Michael F. Toney, Wanli Yang, William E. Gent, Thomas P. Devereaux, Linda F. Nazar, William C. Chueh
Stabilizing high-valent redox couples and exotic electronic states necessitates an understanding of the stabilization mechanism. In oxides, whether they are being considered for energy storage or computing, highly oxidized oxide-anion species rehybridize

Polarization Effects of X-ray Monochromators Modeled Using Dynamical Scattering Theory

July 1, 2021
Author(s)
Marcus Mendenhall, David R. Black, Donald Windover, James Cline
The difference in the diffracted intensity of the sigma-and pi-polarized components of an X-ray beam in powder diffraction has generally been treated according to equations based on dipole scattering, also known as kinematic X-ray scattering. Although this

Two-Dimensional Overdamped Fluctuations of the Soft Perovskite Lattice in CsPbBr 3

July 1, 2021
Author(s)
T. Lanigan-Atkins, X. He, M. Krogstad, D. M. Pajerowski, D. Abernathy, Guangyong Xu, Zhijun Xu, D.-Y. Chung, M. G. Kanatzidis, S. Rosenkranz, R. Osborn, O. Delaire
Lead halide perovskites exhibit structural instabilities and large atomic fluctuations thought to impact their optical and thermal properties, yet detailed structural and temporal correlations of their atomic motions remain poorly understood. Here, these

Freezing of a Disorder Induced Spin Liquid with Strong Quantum Fluctuations

June 29, 2021
Author(s)
Xiao Hu, Daniel M. Pajerowski, Depei Zhang, Andrey Podlesnyak, Yiming Qiu, Qing Huang, Haidong Zhou, Israel Klich, Alexander I. Kolesnikov, M. B. Stone, Seung-Hun Lee
Sr 2CuTe 0.5W 0.5O 6 is a square-lattice magnet with super-exchange between S = 1/2 Cu 2+ spins mediated by randomly distributed Te and W ions. Here, using sub-K temperature and 20 µeV energy resolution neutron scattering experiments we show that this

A Large Beam High Efficiency Radio Frequency Neutron Spin Flipper

June 21, 2021
Author(s)
Wangchun Chen, Ross W. Erwin, Peter Tsai, Md. T. Hassan, Nancy Hadad, Charles F. Majkrzak
A design for a radio-frequency (RF) neutron spin flipper obtained from magneto-static and neutron spin transport simulations is presented. The RF flipper constructed from this design provides a flipping probability of 0.999 or better for a beam size 6 cm

High-Energy Magnetic Excitations from Heavy Quasiparticles in CeCu 2 Si 2

June 18, 2021
Author(s)
Yu Song, Weiyi Wang, Chongde Cao, Zahra Yamani, Yuanji Xu, Yutao Sheng, Wolfgang Loser, Yiming Qiu, Yi-Feng Yang, Robert J. Birgeneau, Pengcheng Dai
The heavy fermion superconductor CeCu 2Si 2 is located near an antiferromagnetic quantum critical point, indicating significant interplay between magnetism and superconductivity. Using inelastic neutron scattering, we show magnetic excitations in CeCu 2Si

Origin and control of ionic hydration patterns in nanopores

June 18, 2021
Author(s)
Miraslau L. Barabash, William A. Gibby, Carlo Guardiani, Alexander Smolyanitsky, Dmitry G. Luchinsky, Peter V. McClintock
In order to permeate a nanopore, an ion must overcome a dehydration energy barrier caused by the redistribution of surrounding water molecules. The redistribution is inhomogeneous, anisotropic and strongly position-dependent, resulting in complex patterns

Monopolar and dipolar relaxation in spin ice Ho2Ti2O7

June 16, 2021
Author(s)
Yishu Wang, T. Reeder, Y. Karaki, J. Kindervater, T. Halloran, Nicholas C. Maliszewskyj, Yiming Qiu, Jose Rodriguez Rivera, Sergiy Gladchenko, S. M. Koohpayeh, S. Nakatsuji, Collin L. Broholm
Ferromagnetically interacting Ising spins on the pyrochlore lattice of corner-sharing tetrahedra form a highly degenerate manifold of low-energy states. A spin flip relative to this "spin-ice" manifold can fractionalize into two oppositely charged magnetic

Database of Ab Initio L-edge X-ray Absorption Near Edge Structure

June 11, 2021
Author(s)
Yiming Chen, Chi Chen, Chen Zheng, Shyam Dwaraknath, Matthew K. Horton, Jordi Cabana, John J. Rehr, John Vinson, Alan K. Dozier, Kristin A. Persson, Shyue P. Ong
The L-edge X-ray Absorption Near Edge Structure (XANES) is widely used in the characterization of transition metal compounds. Here, we report the development of a database of computed L-edge XANES using the multiple scattering theory-based FEFF9 code. The

Field-induced dehydration and optimal ionic escape paths for C2N membranes

June 11, 2021
Author(s)
Miroslav Barabash, William Gibby, Dmitry Luchinsky, Binquan Luan, Alexander Smolyanitsky, Peter McClintock
Most analytic theories describing electrostatically driven ion transport through water-filled nanopores assume that the corresponding permeation barriers are bias-independent. While this assumption may hold for sufficiently wide pores under infinitely

Mobility Extraction in 2D Transition Metal Dichalcogenide Devices - Avoiding Contact Resistance Implicated Overestimation

June 10, 2021
Author(s)
Chin-Sheng Pang, Ruiping Zhou, Xiangkai Liu, Peng Wu, Terry Y. Hung, Shiqi Guo, Mona E. Zaghloul, Sergiy Krylyuk, Albert Davydov, Joerg Appenzeller, Zhihong Chen
Schottky barrier (SB) transistors operate distinctly different from conventional metal-oxide semiconductor field-effect transistors (MOSFETs), in a unique way that the gate impacts the carrier injection from the metal source/drain contacts into the channel
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