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Energy

Alternative energy

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Displaying 101 - 125 of 379

Critical Current Density as a Performance Indicator for Gas-Evolving Electrochemical Devices

August 26, 2020
Author(s)
Jason K. Lee, ChungHyuk Lee, Benzhong Zhao, Jacob LaManna, Eli Baltic, Daniel S. Hussey, David L. Jacobson, Aimy Bazylak
Reaching high current densities is absolutely imperative for electrochemical energy conversion, from fuel cells to CO2 reduction. Here, we identify the existence of a performance indicator for gas-evolving electrochemical energy conversion devices: the

Towards fast screening of organic solar cell blends

August 5, 2020
Author(s)
Lee Richter, Artem Levistsky, Giovanni M. Matrone, Aditi Khirbat, Ilaria Bargigia, Xiaolei Chu, Oded Nahor, Tamar Segal-Perez, Adam Moule, Carlos Silva, Natalie Stingelin, Gitti L. Frey
The ever increasing library of materials systems developed for organic solar-cells, including highly promising non-fullerene acceptors and new, high-efficiency donor polymers, demands the development of methodologies that (i) allow fast screening of a

Understanding Photovoltaic Energy Losses under Indoor Lighting Conditions

July 28, 2020
Author(s)
Behrang H. Hamadani
The external luminescence quantum yield as a function of the solar cell current density when exposed to low indoor light was estimated based on absolute electroluminescence measurements and a self-consistent use of the electro-optical reciprocity

Using Operando Techniques to Understand and Design Alkaline Membrane Fuel Cells with Excellent Performance and Long Operational Stability

July 16, 2020
Author(s)
Xiong Peng, Devashish Kulkarni, Ying Huang, Travis J. Omasta, Benjamin Ng, Yiwei Zheng, Lianqin Wang, Jacob LaManna, Daniel S. Hussey, John R. Varcoe, Iryna V. Zenyuk, William E. Mustain
Operando neutron imaging and operando micro X-ray computed tomography were used to understand the water dynamics of AEMFCs under various operating conditions, and this new fundamental information was used to create electrodes that not only enabled high

Estimation of the critical external heat leading to the failure of lithium-ion batteries

June 29, 2020
Author(s)
Wei Tang, Andy Tam, Liming Yuan, Thomas Dubaniewicz, Richard Thomas, John Soles
A detailed experimental investigation on the critical external heat leading to the failure of lithium-ion (Li-ion) batteries was conducted using an Accelerating Rate Calorimeter (ARC) at the National Institute for Occupational Safety and Health (NIOSH)

Reconciling temperature-dependent factors affecting mass transport losses in polymer electrolyte membrane electrolyzers

June 1, 2020
Author(s)
Jacob LaManna, Aimy Bazylak, ChungHyuk Lee, Jason K. Lee, Kieran F. Fahy, Eli Baltic, Daniel S. Hussey, David L. Jacobson
In this work, we investigated the impact of temperature on two-phase transport in low temperature (LT)-polymer electrolyte membrane (PEM) electrolyzer anode flow channels via in operando neutron imaging and observed a decrease in mass transport

Quasi-elastic Neutron Scattering Measurement of Hydrogen Diffusion in a Graphene Oxide Framework

April 16, 2020
Author(s)
Matthew J. Connolly, Z. N. Buck, Carlos Wexler, Joseph C. Schaeperkoetter, H. Taub, Andrew Gillespie, Helmut Kaiser
We present quasielastic neutron scattering (QENS) spectra from molecular hydrogen adsorbed in GOF. The measurements probed the motion of adsorbed hydrogen as a function of pressure, in order to understand the relationship between the motion of adsorbed

Vibrational Modes and Quantum Zero-Point Energy of Hydrogen in ZrH 0.0155 and ZrH 2

March 25, 2020
Author(s)
Timothy R Prisk, Alexander I. Kolesnikov, Garrett E. Granroth, Jun-li Lin, Brent J. Heuser
We report on an inelastic neutron scattering study of the proton dynamics in ZrH 0.0155 and -ZrHd2^. In particular, we present measurements of the incoherent dynamic structure factor, generalized vibrational density of states, and proton momentum

Chemically Orthogonal Hole Transport Layer for Efficient Colloidal Quantum Dot Solar Cells

March 20, 2020
Author(s)
Margherita Biondi, Min-Jae Choi, Olivier Ouellette, Se-Woong Baek, Petar Todorovi?, Bin Sun, Peicheng Li, Ahmad R. Kirmani, Laxmi Chiluka, Lee J. Richter, Sjoerd Hoogland, Zheng-Hong Lu, F. Pelayo Garc?a de Arquer, Edward H. Sargent, Mingyang Wei
Colloidal quantum dots (CQDs) are of interest in light of their solution-processing and bandgap tuning. Advances in the performance of CQD optoelectronic devices require fine control over the properties of each layer in the device materials stack. This is

Modelling photovoltaic soiling losses through optical characterization

January 9, 2020
Author(s)
Greg P. Smestad, Thomas Germer, Hameed Alrashidi, Eduardo F. Fern?ndez, Sumon Dey, Paidisetty S. Kumar, Honey Brahma, Aritra Ghosh, Nazmi Sellami, Ibrahim A. Hassan, Amal Kasry, Bala Pesala, S. Senthilarasu, Florencia Almonacid, K. S. Reddy, Tapas K. Mallick, Leonardo Micheli
The accumulation of soiling on photovoltaic (PV) modules affects PV systems worldwide. Soiling consists of mineral dust, soot particles, aerosols, pollen, fungi and/or other contaminants that deposit on the surface of PV modules. Soiling absorbs, scatters

Dynamical evolution of the 2D/3D interface: a hidden driver behind perovskite solar cell instability

January 3, 2020
Author(s)
Lee J. Richter, Ahmad R. Kirmani, Albertus A. Sutano, Nikita Drigo, Ines G. Benito, Valentine I. Queloz, Kyung T. Cho, Pascal A. Schouwink, Mohammad K. Nazeeruddin, Giulia Grancini, Sanghyun Paek
Engineering two-/three-dimensional (2D/3D) perovskite solar cells is nowadays a popular strategy for efficient and stable devices. However, the exact function of the 2D/3D interface in controlling the long-term device behavior is still obscure. Here, we

Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites

November 29, 2019
Author(s)
Lee J. Richter, Ahmad R. Kirmani, Xue Wang, Wang Ziyuan, Dinh Cao-Thang, Li Jun, Nam Dae-Hyun, Li Fengwang, Huang Chun-Wei, Tan Chih-Shan, Chen Zitao, Chi Miaofang, Gabardo M. Christine, Seiifitokaldani Ali, Todorovic Petar, Proppe Andrew, Pang Yuanjie, wang yuhang, Ip H. Alexander, Shen-Chuan Lo, shana O. kelley, David Sinton, Edward H. Sargent, Tao-Tao Zhuang, Benjamin Scheffel
The electroreduction of C1 feedgas to high-energy-density fuels provides an attractive avenue to the storage of renewable electricity. Much progress has been made to improve selectivity to C1 and C2 products, however, the selectivity to desirable high

Unveiling defect-mediated charge-carrier recombination at the nanometer scale in polycrystalline solar cells

November 20, 2019
Author(s)
Yohan Yoon, Wei-Chang Yang, Dongheon Ha, Paul M. Haney, Daniel Hirsch, Heayoung Yoon, Renu Sharma, Nikolai Zhitenev
In this work, we employ two techniques, near-field scanning photocurrent microscopy (NSPM) and transmission electron microscope based cathodoluminescence spectroscopy (TEM-CL), to analyze the nanoscale electrical and optical properties of CdTe solar cells

Copper Nanocubes for CO2 Reduction in Gas Diffusion Electrodes

October 31, 2019
Author(s)
Yuxuan Wang, Hao Shen, Ken J. Livi, David Raciti, Han Zong, John Gregg, Mofopefoluwa Onadeko, Yidong Wang, Adam Watson, Chao Wang
Electroreduction of CO2 represents a promising solution for addressing the global challenges in energy and sustainability. The reaction is highly sensitive to the surface structure of electrocatalysts and the local electrochemical environment. We have

HEXRD Measurement of Strain and Dislocation Density ahead of Crack Tips Grown in Hydrogen

September 13, 2019
Author(s)
Matthew J. Connolly, May L. Martin, Peter E. Bradley, Damian S. Lauria, Andrew J. Slifka, Jun Sang Park, Robert Amaro
The deformation fields near fatigue crack tips grown in hydrogen and in air were measured using high-energy x-ray diffraction. A larger magnitude of elastic strain was observed in the hydrogen case compared to the air case. The magnitude of elastic strain

Crystal Orientation Drives the Interface Physics at 2/3-Dimensional Hybrid Perovskites

September 9, 2019
Author(s)
Lee J. Richter, Ahmad R. Kirmani, Marine E. Bouduban, Valentine I. Queloz, Valentina M. Caselli, Kyung T. Cho, Sanghyun Paek, Cristina Roldan-Carmona, Jacques E. Moser, Tom J. Savenije, Mohammad K. Nazeeruddin, Giulia Grancini
Combining halide perovskites with tailored dimensionality into two/three-dimensional (2D/3D) systems has revealed a powerful strategy to boost the performances of perovskite photovoltaics (PVs). Despite recent advances, a clear understanding of the

Engineered Sulfur-MoS2-Graphene Heterostructure Cathodes for Diagnostics of Nanoscale Electrochemical Processes in High Energy Density Li-S Batteries

August 5, 2019
Author(s)
Vladimir P. Oleshko, William R. McGehee, Saya Takeuchi, Siyuan Zhang, Andrei A. Kolmakov, Jabez J. McClelland, Christopher L. Soles
Lithium-sulfur (Li-S) batteries have recently attracted enormous attention because of high theoretical specific energy (2600 Wh kg-1) and high specific capacity (1672 mAhg-1), as well as the low cost, natural abundance, and nontoxicity of elemental sulfur
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