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Daniel S. Hussey, David L. Jacobson, Dusan Spernjak, Adam Weber, Rangachary Mukundan, Joseph Fairweather, Eric Brosha, John Davey, Jacob Spendelow, Rodney Borup
The water sorption of proton-exchange membranes (PEMs) was measured in situ using high-resolution neutron imaging in small-scale fuel-cell test sections. A detailed characterization of the measurement uncertainties and corrections associated with the
Daniel S. Hussey, David L. Jacobson, Chu-lin Cheng, Misun Kang, Juske Horita, sophie voisin, Hassina Bilheux, Warren Jeffery, Edward Perfect
Water retention curves are essential for understanding the hydrologic behavior of partially- saturated porous media and modeling flow transport processes within the vadose zone. In this paper we report direct measurements of the main drying and wetting
Daniel S. Hussey, Han Wen, Huarui Wu, Thomas R. Gentile, Wangchun Chen, David L. Jacobson, Jacob LaManna, B. Khaykovich
Image-forming focusing mirrors were employed to demonstrate two different modalities of neutron imaging, phase imaging with a far-field interferometer, and magnetic-field imaging through the manipulation of the neutron beam polarization. For the phase
Huarui Wu, Zhiyuan Wang, Yao Zhang, Wenbo Mo, Pulin Bai, Kun Song, Zhong Zhang, Zhanshan Wang, Daniel S. Hussey, Yun Liu, Zhe Wang, Xuewu Wang
Neutron-focusing mirrors with both a nested structure and supermirror coatings enable a large collecting area, and consequently a large neutron current gain for mirror-based instruments. A nested neutron-focusing supermirror assembly has been fabricated
Daniel S. Hussey, B. Khaykovich, Jeremy C. Cook, David L. Jacobson, Jacob LaManna, Kiranmayee Kilaru, Brian Ramsey, M. V. Gubarev
The predominate geometry for a neutron imaging experiment is that of a pinhole camera. This is primarily due to the difficulty in focusing neutrons due to the weak refractive index, which is also strongly chromatic. Proof of concept experiments
We present and compare designs of three types of neutron microscopes for high-resolution neutron imaging. Like optical microscopes, our neutron microscopes have both condenser and image-forming objective optics. The optics are based on glancing-incidence
Daniel S. Hussey, Joseph Fairweather, Dusan Spernjak, Adam Weber, David Harvey, Silvia Wessell, David L. Jacobson, Kateryna Artyushkova, Rangachary Mukundan, Rodney Borup
The corrosion of carbon in the electrode supports of proton-exchange-membrane fuel cells leads to electrode collapse, reduced active catalyst area, and increased surface hydrophilicity. While these effects have been linked to performance degradation over
Daniel S. Hussey, Youngju Kim, Jongyul Kim, Seung W. Lee
We introduce an analyzer grating based on a structured scintillator fabricated by a gadolinium oxysulfide powder filling method for a symmetric Talbot-Lau neutron grating interferometer. The analyzer grating, based on a structured scintillator, is an
Daniel S. Hussey, David L. Jacobson, R. A. Winholtz, Hongbin Ma, Corey Borgmeyer, Corey Wilson
An experimental investigation into the parameters affecting heat transport in two three-dimensional oscillating heat pipes (OHP) was implemented. A three-dimensional (3D) OHP is one in which the center axes of the circular channels containing the internal
Neutron radiography enables direct visualization and quantification of many water transport phenomena in proton exchange membrane fuel cells (PEMFCs). The advantage of the technique is that neutrons have a long penetration length through most common PEMFC
Daniel S. Hussey, Jacob LaManna, Eli Baltic, David L. Jacobson
We report on efforts to improve the achievable spatial resolution in neutron imaging by centroiding the scintillation light from gadolinium oxysulfide scintillators. The current state- of-the-art neutron imaging spatial resolution is about 10 µm, and many
Daniel S. Hussey, Muhammad Abir, B. Khaykovich, C. Pfleiderer, Pau Jorba, Marc Seifert, Michael Schulz
We performed spatially resolved imaging of ferromagnetic transitions in Ni3Al and HgCr2Se4 crystals. These neutron depolarization measurements discovered bulk magnetic inhomogeneities in the ferromagnetic transition temperature with the spatial resolution
Micrometer to centimeter scale analyses of the crystalline phase volume fractions in a trip- assisted duplex stainless steel were performed as a function strain using electron backscatter diffraction (EBSD), in situ neutron diffraction, and energy
Daniel S. Hussey, Adam J. Brooks, Caroline G. Lowery, Gerald L. Knapp, Bridget E. Cadigan, Shengmin Guo, Leslie G. Butler
A novel neutron far field interferometer is explored for sub-micron porosity detection in laser sintered SS316 test objects. The results shown are images and volumes of the first quantitative neutron dark-field tomography at various autocorrelation lengths
Daniel S. Hussey, Gary Koenig, Jacob LaManna, David L. Jacobson
Lithium-ion batteries receive significant research effort due to their advantages in energy and power density that is important to enabling many devices. One route to further increase energy density is to fabricate thicker electrodes in the battery cell
Daniel S. Hussey, David L. Jacobson, Hongbin Ma, R. A. Winholtz, Corey Wilson, Corey Borgmeyer
Identical oscillating heat pipes (OHP) charged separately with water and acetone were observed thermally and visually at varying condenser temperatures and heat inputs. Neutron radiography allowed visualization of hydrogen rich liquid water and acetone
Daniel S. Hussey, Jacob LaManna, David L. Jacobson, Gary Koenig
In efforts to increase the energy density of lithium-ion batteries, researchers have attempted to both increase the thickness of battery electrodes and increase the relative fractions of active material. One system that has both of these attributes are
Platinum group metal-free (PGM-free) catalysts are a low-cost alternative to expensive PGM catalysts for polymer electrolyte fuel cells. However, due to the low volumetric activity of PGM-free catalysts, the catalyst layer thickness of the PGM-free
The use of neutron imaging is demonstrated for visualizing and quantifying water content in partially saturated granular porous media. Due to the unique difference in the total neutron cross sections of water, sand and air, a significant contrast for the
Separating acetylene from carbon dioxide is highly challenging but important due to their similar physical properties and molecular dimensions. Capturing carbon dioxide from acetylene by virtue of CO 2-selective absorbents can directly produce pure
D. Campbell, John Collini, J. Slawinska, C. Autieri, L. Wang, K. Wang, B. Wilfong, Y. Eo, Paul Neves, D. Graf, E. Rodriguez, Nicholas Butch, Johnpierre Paglione
Mary Burdette, Beth Armstrong, Ryan Murphy, Luke Heroux, Mathieu Doucet, Stephen Trask, Alexander Rogers, Gabriel Veith
This work probes the slurry architecture of a high silicon content electrode slurry with and without low molecular weight polymeric dispersants as a function of shear rate to mimic electrode casting conditions for poly(acrylic acid) (PAA) and lithium
A robust 2,2'-bipyridine (bpy)-derived biological hydrogenbonded framework (HOF-25) has been realized depending on guanine-quadruplex with the assistance of π-π interaction, which reacts with Re(CO) 5Cl to give a post-functionalized HOF-25-Re. Xray
Yanqin Zhai, Nicos Martys, William L. George, Joseph E. Curtis, Jannatun Nayem, Y. Z, Yun Liu
In the past decade, there is increased research interest in studying internal motions of flexible proteins in solution using Neutron Spin Echo (NSE) as NSE can simultaneously probe the dynamics at the length and time scale comparable to protein domain
Rahul Chadda, Nathan Bernhardt, Elizabeth Kelley, Susana Marujo Teixeira, Kacie Griffith, Alejandro Gil-Ley, Tugba Ozturk, Lauren Hughes, Ana Forsythe, Venkatramanan Krishnamani, Jose Faraldo-Gomez, Janice Robertson
Over two-thirds of integral membrane proteins of known structure assemble into oligomers. Yet, the forces that drive the association of these proteins remain to be delineated, as the lipid bilayer is a solvent environment that is both structurally and