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Search Publications by: Collin L. Broholm (Assoc)

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Displaying 1 - 25 of 35

Continuum of magnetic excitations in the Kitaev honeycomb iridate D3LiIr2O6

February 12, 2024
Author(s)
Thomas Halloran, Yishu Wang, Kemp Plumb, M. B. Stone, Barry Winn, M. K. Graves-Brook, Jose Rodriguez Rivera, Yiming Qiu, Prashant Chauhan, N. Armitage, Tomohiro Takayama, Hidenori Takagi, Collin L. Broholm
Inelastic neutron scattering (INS) measurements of powder D3(7Li)(193Ir)2O6 reveal low energy magnetic excitations with a scattering cross section that is featureless versus |Q| and consistent with a Kitaev spin-liquid (KSL) state. The magnetic nature of

Noncollinear 2k Antiferromagnetism in the Zintl Semiconductor Eu5In2Sb6

January 29, 2024
Author(s)
Vincent Morano, Jonathan N. Gaudet, Nicodemos Varnava, Tanya Berry, Thomas Halloran, Chris Lygouras, Xiaoping Wang, Christina M. Hoffman, Guangyong Xu, Jeffrey Lynn, Tyrel McQueen, David Vanderbilt, Collin L. Broholm
Eu5In2Sb6 is an orthorhombic non-symmorphic small band gap semiconductor with three distinct Eu2+ sites and two low-temperature magnetic phase transitions. The material displays one of the greatest (negative) magnetoresistances of known stoichiometric

Spin-orbital order and excitons in magnetoresistive HoBi

March 22, 2023
Author(s)
Jonathan N. Gaudet, H. Yang, E. Smith, T. Halloran, J. Clancy, Jose Rodriguez Rivera, Guangyong Xu, Yang Zhao, Wangchun Chen, G. Sala, Adam A. Aczel, B. Gaulin, Fazel Tafti, Collin L. Broholm
The magnetism of the rock-salt fcc rare-earth monopnictide HoBi, a candidate topological material with extreme magnetoresistance, is investigated. From the Ho3+ non-Kramers J=8 spin-orbital multiplet, the cubic crystal electric field yields six near

Geometrical Frustration Versus Kitaev Interactions in BaCo 2 (AsO 4 ) 2

January 10, 2023
Author(s)
Thomas Halloran, Felix Desrochers, Emily Zhang, Tong Chen, Li E. Chern, Zhijun Xu, Barry Winn, Melissa Graves-Brook, M. B. Stone, Alexander I. Kolesnikov, Yiming Qiu, Ruidan Zhong, Robert Cava, Yong Kim, Collin L. Broholm
Recently, Co-based honeycomb magnets have been proposed as promising candidate materials to host the Kitaev spin liquid state. One of the front-runners is BaCo 2(AsO 4) 2 (BCAO), where it was suggested that the exchange processes between Co 2+ ions via the

Weyl-mediated helical magnetism in NdAlSi

August 19, 2021
Author(s)
Jonathan Gaudet, Hung-Yu Yang, Santu Baidya, Baozhu Lu, Guangyong Xu, Yang Zhao, Jose Rodriguez Rivera, Christina M. Hoffman, David E. Graf, Darius H. Torchinsky, Predrag Nikolic, David Vanderbilt, Fazel Tafti, Collin L. Broholm
Emergent relativistic quasiparticles in Weyl semimetals are the source of exotic electronic properties such as surface Fermi arcs, the anomalous Hall effect and negative magnetoresistance, all observed in real materials. Whereas these phenomena highlight

Monopolar and dipolar relaxation in spin ice Ho2Ti2O7

June 16, 2021
Author(s)
Yishu Wang, T. Reeder, Y. Karaki, J. Kindervater, T. Halloran, Nicholas C. Maliszewskyj, Yiming Qiu, Jose Rodriguez Rivera, Sergiy Gladchenko, S. M. Koohpayeh, S. Nakatsuji, Collin L. Broholm
Ferromagnetically interacting Ising spins on the pyrochlore lattice of corner-sharing tetrahedra form a highly degenerate manifold of low-energy states. A spin flip relative to this "spin-ice" manifold can fractionalize into two oppositely charged magnetic

Pristine Quantum Criticality in a Kondo Semimetal

May 19, 2021
Author(s)
Wesley T. Fuhrman, Andrey Sidorenko, Jonathan Hanel, Hannes Winkler, Andrey Prokofiev, Jose Rodriguez Rivera, Yiming Qiu, Peter Blaha, Qimiao Si, Collin L. Broholm, Silke Paschen
The observation of quantum criticality in diverse classes of strongly correlated electron systems has been instrumental in establishing ordering principles, discovering new phases, and identifying the relevant degrees of freedom and interactions. At focus

Noncollinear Ferromagnetic Weyl Semimetal with Anisotropic Anomalous Hall Effect

March 24, 2021
Author(s)
Hung-Yu Yang, Bahadur Singh, Jonathan Gaudet, Baozhu Lu, Cheng-Yi Huang, Wei-Chi Chiu, Shin-Ming Huang, Baokai Wang, Faranak Bahrami, Bochao Xu, Jacob Franklin, Ilya Sochnikov, David Graf, Guangyong Xu, Yang Zhao, Christina Hoffman, Hsin Lin, Darius Torchinsky, Collin L. Broholm, Arun Bansil, Fazel Tafti

Multiphase Magnetism in Yb 2 Ti 2 O 7

November 3, 2020
Author(s)
Allen Scheie, Jonas Kindervater, Shu Zhang, Hitesh Changlani, G. Sala, Georg Ehlers, Andre Heinemann, Gregory Tucker, Seyed Koohpayeh, Collin L. Broholm

Antichiral Spin Order, its Soft Modes, and their Hybridization with Phonons in the Topological Semimetal Mn 3 Ge

August 3, 2020
Author(s)
Y. Chen, Jonathan Gaudet, S. Dasgupta, G. G. Marcus, J. Lin, T. Chen, T. Tomita, M. Ikhlas, Yang Zhao, Wangchun Chen, Matthew B. Stone, O. Tchernyshyov, S. Nakatsuji, Collin L. Broholm
Quantum materials with strong transport responses to disparate physical quantities are of great fundamental significance and may hold technological potentials. The interplay between interactions and topology drive such responses through the effects of

Orientation Dependence of the Magnetic Phase Diagram of Yb 2 Ti 2 O 7

May 21, 2020
Author(s)
S. Saubert, A. Scheie, C. Duvinage, J. Kindervater, S. Zhang, H. J. Changlani, Guangyong Xu, S. M. Koohpayeh, O. Tchernyshyov, Collin L. Broholm, C. Pfleiderer
In the quest to realize a quantum spin liquid (QSL), magnetic long-range order is hardly welcome. Yet it can offer deep insights into a complex world of strong correlations and fluctuations. Much hope was placed in the cubic pyrochlore Yb 2Ti 2O 7 as a

Anisotropic Effect of a Magnetic Field on the Neutron Spin Resonance in FeSe

April 16, 2020
Author(s)
Tong Chen, Youzhe Chen, David W. Tam, Bin Gao, Yiming Qiu, Astrid Schneidewind, Igor Radelytskyi, Karel Prokes, Songxue Chi, Masaaki Matsuda, Collin L. Broholm, Pengcheng Dai
We use inelastic neutron scattering to study the effect of a magnetic field on the neutron spin resonance (Er = 3.6 meV) of superconducting FeSe (Tc = 9 K). While a field aligned along the in-plane direction broadens and suppresses the resonance, a c-axis

Low-Energy Magnons in the Chiral Ferrimagnet Cu 2 OSeO 3 : A Coarse-Grained Approach

April 8, 2020
Author(s)
Yi Luo, G. G. Marcus, Benjamin Trump, J. Kindervater, M. B. Stone, Jose Rodriguez Rivera, Yiming Qiu, T. M. McQueen, O. Tchernyshyov, Collin L. Broholm
We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic Cu 2OSeO 3. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic configuration of the "strong

Homogeneous Reduced Moment in a Gapful Scalar Chiral Kagome Antiferromagnet

July 12, 2019
Author(s)
A. Scheie, S. Dasgupta, M. Sanders, A. Sakai, Y. Matsumoto, Timothy R Prisk, S. Nakatsuji, R. J. Cava, Collin L. Broholm
We present a quantitative experimental investigation of the scalar chiral magnetic order with in Nd 3Sb 3Mg 2O 14. Static magnetization reveals a net ferromagnetic ground state, and inelastic neutron scattering from the hyperfine coupled nuclear spin

Anisotropic Spin Fluctuations in Detwinned FeSe

July 1, 2019
Author(s)
Tong Chen, Youzhe Chen, Andreas Kreisel, Xingye Lu, Astrid Schneidewind, Yiming Qiu, J. T. Park, Toby G. Perring, J. Ross Stewart, Huibo Cao, Rui Zhang, Yu Li, Yan Rong, Yuan Wei, Brian M. Andersen, P. J. Hirschfeld, Collin L. Broholm, Pengcheng Dai
Superconductivity in iron selenide (FeSe) emerges from a nematic phase that breaks four-fold rotational symmetry in the iron plane [Fig. 1(a)] [1-4]. Although this phase in FeSe is established below a tetragonal-to-orthorhombic transition temperature Τ s

Incommensurate Magnetism near Quantum Criticality in CeNiAsO

May 15, 2019
Author(s)
Shan Wu, W. A. Phelan, L. Liu, J. R. Morey, J. A. Tutmaher, J. C. Neuefeind, Ashfia Huq, Matthew B. Stone, M. Feygenson, David W. Tam, Benjamin A. Frandsen, Benjamin Trump, Cheng Wan, S. R. Dunsiger, Tyrel M. McQueen, Y. J. Uemura, Collin L. Broholm

Continuum of Quantum Fluctuations in a Three-Dimensional S = 1 Heisenberg Magnet

January 1, 2019
Author(s)
K. W. Plumb, Hitesh J. Changlani, A. Scheie, Shu Zhang, J. W. Krizan, Jose Rodriguez Rivera, Yiming Qiu, B. Winn, R. J. Cava, Collin L. Broholm
Spin liquids are a fundamentally new phase of matter that cannot be described by a broken symmetry and have no order parameter. While the quantum entanglement that characterizes a quantum spin liquid is not directly accessible to any current measurement

Screened Moments and Extrinsic In-Gap States in Samarium Hexaboride

April 18, 2018
Author(s)
W. T. Fuhrman, J. R. Chamorro, P. A. Alekseev, J.-M. Mignot, T. Keller, Jose Rodriguez Rivera, Yiming Qiu, P. Nikolic, T. M. McQueen, Collin L. Broholm
The Kondo impurity effect in metals is the result of quantum-mechanical scattering of conduction electrons by magnetic impurities. 1 This process leads to exotic effects such as unconventional superconductivity and an effective electron mass enhanced by 2

Reentrant Phase Diagram of Yb 2 Ti 2 O 7 in a [111] Magnetic Field

September 22, 2017
Author(s)
A. Scheie, J. Kindervater, S. Saubert, C. Duvinage, C. Pfleiderer, H. J. Changlani, S. Zhang, Leland Harriger, K. Arpino, S. M. Koohpayeh, Collin L. Broholm
We present a phase diagram of rare-earth pyrochlore Yb 2Ti 2O 7 in a (111) magnetic field. Using heat capacity, magnetization, and neutron scattering data, we show an unusual field-dependence of a first-order phase boundary, wherein a small applied field

Gapped Excitations in the High-Pressure Antiferromagnetic Phase of URu 2 Si 2

May 31, 2017
Author(s)
T. J. Williams, H. Barath, Z. Yamani, Jose Rodriguez Rivera, Juscelino Leao, J. D. Garrett, G. M. Luke, W.J. L. Buyers, Collin L. Broholm
We report a neutron scattering study of the magnetic excitation spectrum in each of the three temperature and pressure phases of URu 2Si 2. We find qualitatively similar excitations throughout the (H0L)scattering plane in the hidden order and large moment

Spin Excitations and the Fermi Surface of Superconducting FeS

March 10, 2017
Author(s)
Haoran Man, Jiangang Guo, Rui Zhang, Rico U. Schonemann, Zhiping Yin, Mingxuan Fu, Matthew B. Stone, Qingzhen Huang, Yu Song, Weiyi Wang, David J. Singh, Felix Lochner, Tillman Hickel, Ilya Eremin, Leland Harriger, Jeffrey W. Lynn, Collin L. Broholm, Luis Balicas, Qimiao Si, Pengcheng Dai

Disordered Route to the Coulomb Quantum Spin Liquid: Random Transverse Fields on Spin Ice in Pr 2 Zr 2 O 7

March 8, 2017
Author(s)
J.-J. Wen, S.M. Koohpayeh, K. A. Ross, B. A. Trump, T. M. McQueen, K. Kimura, S. Nakatsuji, Yiming Qiu, D. M. Pajerowski, John R. Copley, Collin L. Broholm
Inelastic neutron scattering reveals a broad continuum of excitations in Pr 2Zr 2O 7, the temperature and magnetic field dependence of which indicate a continuous distribution of quenched transverse fields (Δ}) acting on the non-Kramers Pr 3+ crystal

Modulated Magnetism and Anomalous Electronic Transport in Ce 3 Cu 4 As 4 O 2

August 29, 2016
Author(s)
Jiakui K. Wang, Shan Wu, Yiming Qiu, Jose Rodriguez Rivera, Qingzhen Huang, Collin L. Broholm, E. Morosan
The complex magnetism and transport properties of tetragonal Ce 3Cu 4As 4O 2 were examined through neutron scattering and physical properties measurements on polycrystalline samples. The lamellar structure consists of alternating layers of CeCu 4As 4 with

Modulated Magnetism and Anomalous Electronic Transport in Ce 3 Cu 4 As 4 O 2

August 29, 2016
Author(s)
Jiakui K. Wang, Shan Wu, Yiming Qiu, Jose Rodriguez Rivera, Qingzhen Huang, Collin L. Broholm, E. Morosan
The complex magnetism and transport properties of tetragonal Ce 3Cu 4As 4O 2 were examined through neutron scattering and physical properties measurements on polycrystalline samples. We find a lamellar structure consisting of alternating layers of CeCu 4As