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Large Magnetic Susceptibility Anisotropy of Metallic Carbon Nanotubes
Published
Author(s)
Jeffrey A. Fagan, Erik K. Hobbie, Jun Kono, Thomas Searles, Y Imanaka, T Takamasu, H Ajiki
Abstract
Through magnetic linear dichroism spectroscopy, the magnetic susceptibility anisotropy of metallic single-walled carbon nanotubes has been extracted and found to be 2-4 times greater than values for semiconducting single-walled carbon nanotubes. This large anisotropy is consistent with our calculations and can be understood in terms of large orbital paramagnetism of electrons in metallic nanotubes arising from the Aharonov-Bohm-phase-induced gap opening in a parallel ¯eld. We also compare our values with previous work for semiconducting nanotubes, which con¯rm a break from the prediction that the magnetic susceptibility anisotropy increases linearly with the diameter.
Fagan, J.
, Hobbie, E.
, Kono, J.
, Searles, T.
, Imanaka, Y.
, Takamasu, T.
and Ajiki, H.
(2010),
Large Magnetic Susceptibility Anisotropy of Metallic Carbon Nanotubes, Physical Review Letters, [online], https://doi.org/10.1103/PhysRevLett.105.017403
(Accessed October 14, 2025)