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Recent literature reports of transient infrared hole-burning and spectroscopic measurements on water and ice are critically reviewed. Dynamical measurements on the femtosecond and picosecond timescales show anomalous vibrational relaxation temperature dependencies and crystalline-like structures that are identified within the inhomogeneous hydroxyl-stretching band of both water phases.
Citation
Science
Volume
283
Pub Type
Journals
Keywords
hydrogen bonding, ice, infrared, molecular dynamics, temperature dependence, transient IR spectroscopy, ultrafast, vibrational lifetime
Citation
Heilweil, E.
(1999),
Ultrafast Glimpses at Water and Ice, Science
(Accessed June 4, 2023)