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Christopher L. Soles, Kanae N. Ito, Adam B. Burns, Edwin P. Chan, Robert M. Dimeo, Madhu Sudan Tyagi, Albert F. Yee, Jianwei Liu
This article explores the relationship between the nano- to picosecond dynamics, as quantified by elastic incoherent neutron scattering, in polycarbonate (PC) glasses with their mechanical toughness. We establish a robust correlation between mechanical
Xiong Peng, Devashish Kulkarni, Ying Huang, Travis J. Omasta, Benjamin Ng, Yiwei Zheng, Lianqin Wang, Jacob LaManna, Daniel S. Hussey, John R. Varcoe, Iryna V. Zenyuk, William E. Mustain
Operando neutron imaging and operando micro X-ray computed tomography were used to understand the water dynamics of AEMFCs under various operating conditions, and this new fundamental information was used to create electrodes that not only enabled high
Dominik P. Halter, Ryan Klein, Michael A. Boreen, Benjamin Trump, Craig Brown, Jeffrey R. Long
A new, air-stable, permanently porous uranium(IV) metal–organic framework U(bdc) 2 (1, bdc 2− = 1,4-benzenedicarboxylate) was synthesized and its H 2 and CH 4 adsorption properties were investigated. Low temperature adsorption isotherms confirm strong
Y.- Y. Jau, Wangchun Chen, Thomas R. Gentile, Daniel S. Hussey
We report an experimental implementation for neutron transverse polarization analysis that is able to detect a small angular change (10^-3 rad) of neutron spin orientation and works for both monochromatic and polychromatic neutron beams. Our approach
Erkan Senses, Saeid Darvishi, Madhu Sudan Tyagi, Antonio Faraone
We investigate single chain dynamics of an entangled linear poly (ethylene oxide) melt in presence of well-dispersed attractive nanoparticles using high resolution neutron spectroscopy at particle volume fractions as high as 0.53. The short time dynamics
The symmetric geometry of a grating interferometer is advantageous because it gives a maximum phase-sensitivity when the sample is at the phase grating position. However, the spatial resolution is reduced due to the geometric blur due to the increased
Frank Heinrich, Paul Kienzle, David P. Hoogerheide, Mathias Loesche
We apply a framework to quantify information gain from neutron or x-ray reflectometry experiments (Treece et al., 2019), in an in-depth investigation into the design of scattering contrast in biological and soft matter surface architectures. To focus the
John M Jurns, Michael Middleton, Robert E. Williams
The NIST Center for Neutron Research (NCNR) operates a 20 MW research reactor that produces neutrons for a suite of 30 neutron scattering instruments. 70% of these instruments use cold neutrons (E 2), which is in turn cooled by a recently commissioned 7 kW
Shyam S. Mohapatra, Robert D. Frisina, Subhra Mohapatra, Kevin B. Sneed, Eleni Markoutsa, Tao Wang, Rinku Dutta, Ratka Damnjanovic, Manh-Huong Phan, Daniel J. Denmark, Manas R. Biswal, Andrew R. McGill, Ryan Green, Mark Howell, Payal Ghosh, Alejandro Gonzalez, Nadia Tasnim Ahmed, Brittney Borresen, Mitchell Farmer, Melissa Gaeta, Krishna Sharma, Christen Bouchard, Danielle Gamboni, Jaime Martin, Bianca Tolve, Mandip Singh, Jack W. Judy, Chenzhong Li, Swadeshmukul Santra, Sylvia Daunert, Elnaz Zeynaloo, Ryan M. Gelfand, Steven Lenhert, Eric S. McLamore, Dong Xiang, Victoria Morgan, Lisa E. Friedersdorf, Ratnesh Lal, Thomas J. Webster, David Hoogerheide, Thanh Duc Nguyen, Martin J. D'Souza, Mustafa Culha, Pierre P. Kondiah, Donald K. Martin
Whitney S. Loo, Antonio Faraone, Lorena S. Grundy, Kevin W. Gao, Nitash P. Balsara
Polymer chain dynamics of a nanostructured block copolymer electrolyte are investigated by neutron spin-echo spectroscopy. Monomeric friction, determined by fitting the short-time data to the Rouse model, increases with increasing salt concentration. Tube
PROSPECT COLLABORATION, Jerome LaRosa, Hans Pieter Mumm, Svetlana Nour, Mark Tyra, Denis E. Bergeron
Reactor neutrino experiments have seen major improvements in precision in recent years. With the experimental uncertainties starting to surpass those from theory, it is important to carefully consider all sources of e in making theoretical predictions
David P. Hoogerheide, Philip A. Gurnev, Tatiana K. Rostovtseva, Sergey M. Bezrukov
Post-translational modifications (PTMs) of proteins are recognized as crucial components of cell signaling pathways through modulating folding, altering stability, changing interactions with ligands, and, therefore, serving multiple regulatory functions
Maria Papachristodoulou, James Doutch, Hoi Sang Beatrice Leung, Andy Church, Thomas Charleston, Luke A. Clifton, Paul Butler, Christopher J. Roberts, Daniel G. Bracewell
A deeper understanding of the nano and mesoscale structure of chromatographic adsorbents and the distribution of proteins within the media, is critical to a mechanistic understanding of separation processes using these materials. Characterisation of the
Development of high-performance and cost-effective catalysts is pivotal to render hydrazine monohydrate (N 2H 4.H 2O) viable as a hydrogen carrier. Herein, we report a detailed study on development of noble-metal-free Ni–W–O derived nanocomposite catalysts
Mihee Kim, Frank Heinrich, Greg Haugstad, Guichuan Yu, Guangcui Yuan, Sushil K. Satija, Wenjia Zhang, Hannah S. Seo, Joseph M. Metzger, Samira M. Azarin, Timothy P Lodge, Benjamin J. Hackel, Frank S. Bates
Maintaining the integrity of cell membranes is indispensable for cellular viability. Poloxamer 188 (P188), a poly(ethylene oxide)-b-poly(propylene oxide)-b-poly(ethylene oxide) (PEO-PPO-PEO) triblock copolymer with a number average molecular weight of 8
Duncan H. Moseley, Shelby E. Stavretis, Zhenhua Zhu, Mei Guo, Craig Brown, Mykhaylo Ozerov, Yongqiang Cheng, Luke L. Daemen, Rachael Richardson, Gary Knight, Komalavalli Thirunavukkuarasu, Anibal J. Ramirez-Cuesta, Jinkui Tang, Zi-Ling Xue
Spin-phonon coupling plays a critical role in magnetic relaxation in single-molecule magnets (SMMs) and molecular qubits. Yet, few studies of its nature have been conducted. Phonons here refer to both intermolecular and intramolecular vibrations. In the
Bao Qiu, Minghao Zhang, Seung-Yong Lee, Haodong Liu, Thomas A. Wynn, Lijun Wu, Yimei Zhu, Wen Wen, Craig Brown, Dong Zhou, Zhaoping Liu, Ying Shirley Meng
Great focus has been placed on the advancement of anionic redox, to which Li-rich layered oxide cathodes high capacities - currently exceeding 300 mAh g -1 - are attributed. With almost doubled capacity compared with present cathode materials, performance
Vivek M. Prabhu, Kenneth Mineart, Guangmin Wei, James Hedrick, Yi Yan Yang, Shrinivas Venkataraman
The cholesterol-functionalized polycarbonate-based diblock copolymer, PEG113-b-P(MTC-Chol)30, forms pathway-dependent nanostructures via dialysis-based solvent exchange. The initial organic solvent that dissolves or disperses the polymer dictates a self
The relationship between the membrane bending modulus (k) and compressibility modulus (KA) depends on the extent of coupling between the two monolayers (leaflets). Using neutron spin echo (NSE) spectroscopy, we investigate the effects of n-alkanes on the
Anthony J. Campanella, Benjamin Trump, Eric J. Gosselin, Eric D. Bloch, Craig Brown
Metal-organic frameworks featuring open metal coordination sites have been widely studied for the separation of gas mixtures. For CO 2/N 2 separations, these materials have shown considerable promise. Herein, we report the characterization of a subset of
Tingting Liu, Siddharth Guatam, David R. Cole, Sumant Patankar, David Tomasko, Wei Zhou, Gernot Rother
Fundamental understanding of subcritical/supercritical behavior of key hydrocarbon species inside nanoporous matrices at elevated pressure and temperature is less developed compared to bulk fluids, but this knowledge is needed for efficient utilization of
Q Liu, M Febbraro, R.J. deBoer, S. Aguilar, A Boeltzig, Y Chen, M Couder, J Gorres, Jamie Weaver, K. T. Macon, M. Wiescher, K. Manukyan, L. Morales, S Pain, W. A. Peters, C. Seymour, G. Seymour, R. Toomey, B. Vande Kolk
Nucleosynthesis in the fi rst generation of massive stars offer a unique setting to explore the creation of the fi rst heavier nuclei in an environment free of impurities from earlier stellar generations. In later generations of massive stars, hydrogen