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A facile method in synthesizing crystalline lithiated amines via ball milling primary amines with LiH unprecedented endothermic dehydrogenation feature in the temperature range of 150-250 Degree}C., showing potentials as a new type of hydrogen storage material. Structural analysis and mechanistic studies on lithiated ethylenediamine (li2EDA) indciate that LI may mediate the dehyrodgenation through α, β LiH elimination mechanism, creating a more energy favorable pathway for the selective H2 release.
Chen, J.
, Wu, H.
, Wu, G.
, Xiong, Z.
, Wang, R.
, Fan, H.
, Zhou, W.
, Liu, B.
, Chua, Y.
, Ju, X.
and Chen, P.
(2014),
Lithiated Primary Amine-A New Material for Hydrogen Storage, Chemistry-A European Journal, [online], https://tsapps.nist.gov/publication/get_pdf.cfm?pub_id=915795
(Accessed October 10, 2025)