, B.
, , J.
, , A.
, , M.
, Kim, J.
, Qiu, Y.
, Copley, J.
, Schiffer, P.
and Cava, R.
(2010),
Coexisting Magnetic Order and Cooperative Paramagnetism in the Stuffed Pyrochlore Tb<sub>2+x</sub>Ti<sub>2-2x</sub>Nb<sub>x</sub>O<sub>7</sub>, Physical Review Letters
(Accessed October 20, 2025)
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Coexisting Magnetic Order and Cooperative Paramagnetism in the Stuffed Pyrochlore Tb2+xTi2-2xNbxO7
Published
Author(s)
, , A. J. Williams, M. L. Dahlberg, J.G. Kim, , , P. Schiffer, R J. Cava
Abstract
Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, cooperative paramagnetic behavior exists for all x, and for Tb3NbO7 an antiferromagnetically ordered state coexists with cooperative paramagnetic behavior, without applying any external fields or pressure. These results are a new thrust into the study of spin liquids and cooperative paramagnets, opening a new route to study this unique cooperative behavior.Citation
Physical Review Letters
Volume
81
Issue
6
Pub Type
Journals
Keywords
Magnetic frustration, spin liquid, antiferromagnetic order
Citation
Issues
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Created February 18, 2010, Updated February 19, 2017