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Search Publications by: Lucas Flagg (Fed)

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Displaying 1 - 10 of 10

New Method to Probe the Surface Properties of Polymer Thin Films by Two-Dimensional (2D) Inverse Gas Chromatography (iGC)

June 25, 2024
Author(s)
Whirang Cho, Lucas Flagg, Christopher Stafford, Jeremiah Woodcock, Daniel Burnett, Anett Kondor, Douglas Fox, John Hoffmann
Polymer-based functional surface coatings are extensively used in advanced technologies, including optics, energy, and environmental applications. Surface thermodynamic properties profoundly impact the molecular interactions that control interfacial

Trace Water Effects on Crystalline 1-Ethyl-3-methylimidazolium Acetate

May 16, 2023
Author(s)
Ashlee Aiello, John Hoffman, Anthony Kotula, Lucas Flagg, Ruipeng Li, Jeremiah Woodcock
Spontaneous room temperature crystallization of 1-ethyl-3-methylimidazolium acetate ([C2mim][OAc]) was observed upon removal of trace water. To ensure that this observation was not produced by trace water or other contaminants, sample purity was confirmed

Salts as additives: A route to improve performance and stability of n-type organic electrochemical transistors

March 9, 2023
Author(s)
David Ohayon, Lucas Flagg, Andrea Giugni, Shofarul Wustoni, Ruipeng Li, Tania Hidalgo, Abdul Hamid Emwas, Rajendar Sheelamanthula, Iain McCulloch, Lee J. Richter, Sahika Inal
Organic electrochemical transistors (OECTs) are becoming increasingly ubiquitous in a wide variety of applications at the interface with biological systems, including biosensing, neuromorphic computing, and logic circuits. The widespread use of these

Quantitative relationships between film morphology, charge carrier dynamics, and photovoltaic performance in bulk-heterojunction binary vs. ternary acceptor blends

February 7, 2023
Author(s)
Weigang Zhu, Guoping Li, Subhrangsu Mukherjee, Natalia Powers-Riggs, Leighton Jones, Eliot Gann, R Joseph Kline, Andrew Herzing, Jenna Logsdon, Lucas Flagg, Charlotte Stern, Ryan Young, Kevin Kohlstedt, George Schatz, Dean DeLongchamp, Michael Wasielewski, Ferdinand Melkonyan, Antonio Facchetti, Tobin Marks
Addressing pertinent and perplexing questions regarding why nonfullerene acceptors (NFAs) promote higher power conversion efficiencies (PCEs) than traditional fullerenes and how photoactive bulk heterojunction (BHJ) film morphology, charge photogeneration

Hydration of a side-chain-free n-type ladder semiconducting polymer driven by electrochemical doping

January 11, 2023
Author(s)
Jiajie Guo, Lucas Flagg, Duyen Tran, Shinya Chen, Ruipeng Li, Nagesh Kolhe, Rajiv Giridharagopal, Samson A. Jenekhe, Lee J. Richter, David Ginger
We study the organic electrochemical transistor (OECTs) performance of the ladder polymer, poly(benzimidazobenzophenanthroline) (BBL) in an attempt to better understand how an apparently insoluble side-chain free polymer is able to operate as an OECT with

In-situ studies of the swelling by electrolyte in the electrochemical doping of an ethylene glycol substituted polythiophene

June 13, 2022
Author(s)
Lee J. Richter, Lucas Flagg, Lauren Asselta, Nicholas D'Antona, Natalie Stingelin, Tommaso Nicolini, Jonathan Onorato, Christine Luscombe, Ruipeng Li
Organic mixed ionic electronic conductors (OMIECs) have the potential to enable diverse new technologies, ranging from biosensors to flexible energy storage devices and neuromorphic computing platforms. However, study of these materials in their operating

Impact of Varying Side Chain Structure on Organic Electrochemical Transistor Performance: A Series of Oligoethylene Glycol-substituted Polythiophenes

April 19, 2022
Author(s)
Shinya Chen, Lucas Flagg, Jonathan Onorato, Lee J. Richter, Christine Luscombe, David Ginger
We study the electrochemical doping/dedoping kinetics, and the organic electrochemical transistor (OECT) performance of a series polythiophene homopolymers with ethylene glycol units in their side chains using both kosmotropic and chaotropic anion

Side Chain Engineering Control of Mixed Conduction in Oligoethylene Glycol-Substituted Polythiophenes

August 31, 2021
Author(s)
Jonathan Onorato, Zhongyang Wang, Yangyang Sun, Christian Nowak, Ban Dong, Lucas Flagg, Ruipeng Li, Lee J. Richter, Fernando Escobedo, Paul Nealey, Shrayesh Patel, Christine Luscombe
A major limitation for polymeric mixed ionic/electronic conductors (MIECs) is the trade-off between ionic and electronic conductivity; changes made that improve one typically hinder the other. In order to address this fundamental problem, this work