NIST Authors in Bold
| Author(s): | Douglas T. Smith; Jon R. Pratt; Francesca M. Tavazza; Lyle E. Levine; Anne M. Chaka; |
|---|---|
| Title: | An Ultra-Stable Platform for the Study of Single-Atom Chains |
| Published: | May 16, 2010 |
| Abstract: | We describe a surface probe instrument capable of sustaining single-atomic-bond junctions in the electronic quantum-conduction regime for tens of minutes, and present results for Au junctions that can be locked stably in n = 1 and n = 2 quantum conduction states with electrical conductivity nG0 (G0 = 2e2/h) and switched in a controlled way. The instrument measures and controls the gap formed between a probe and a flat surface with better than 5 pm long-term stability in a high-vacuum chamber at 4 K using a high-sensitivity fiber-optic interferometer that forms a Fabry-Perot cavity immediately adjacent and parallel to the probe. We also report the experimental observation of stable non-integer conduction states, along with preliminary density-functional-theory-based calculations of one-dimensional and two-dimensional Au bridges that also produce non-integer conduction states. Finally, we report the observation of novel stochastic processes related to non-ballistic electron transport through strained single-atomic-bond junctions. The instrument permits detailed study of electron transport in one-dimensional systems, and the long-term picometer stability of the junction holds great promise for application to single-molecule spectroscopy. |
| Citation: | Journal of Applied Physics |
| Volume: | 107 |
| Pages: | 5 pp. |
| Keywords: | nanomechanics; quantized conductance; nanowire; single atom chain; interferometry |
| Research Areas: | Nanostructures |